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Dynamic Stark Control of Photochemical Processes
Abstract
A method is presented for controlling the outcome of photochemical reactions by using the dynamic Stark effect due to a strong, nonresonant infrared field. The application of a precisely timed infrared laser pulse reversibly modifies potential energy barriers during a chemical reaction without inducing any real electronic transitions. Dynamic Stark control (DSC) is experimentally demonstrated for a nonadiabatic photochemical reaction, showing substantial modification of reaction channel probabilities in the dissociation of IBr. The DSC process is nonperturbative and insensitive to laser frequency and affects all polarizable molecules, suggesting broad applicability.
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Citations
Cited by
Krausz, F., & Ivanov, M. (2009) · Reviews of Modern Physics · doi:10.1103/revmodphys.81.163 · Cited by 5,468
Self-citationLoh, Z.-H., & Leone, S. R. (2013) · The Journal of Physical Chemistry Letters · doi:10.1021/jz301910n · Cited by 66
Metadata
- Authors
- Sussman, B. J., Townsend, D., Ivanov, M. Y., & Stolow, A.
- Venue
- Science
- Published
- 2006-10-13
- Volume
- 314
- Issue
- 5797
- Pages
- 278-281
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2081407315
- Cited by
- 363
- References
- 0
- FWCI
- 11.81
- Type
- journal article
- Language
- en
- Open access
- closed
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- Sussman, B. J., Townsend, D., Ivanov, M. Y., & Stolow, A. (2006). Dynamic Stark Control of Photochemical Processes. Science. https://doi.org/10.1126/science.1132289
Data sources
Bibliographic data: Semantic Scholar, OpenAlex, Crossref.
Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
