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Photoconductive Coaxial Nanotubes of Molecularly Connected Electron Donor and Acceptor Layers
Abstract
Controlled self-assembly of a trinitrofluorenone-appended gemini-shaped amphiphilic hexabenzocoronene selectively formed nanotubes or microfibers with different photochemical properties. In these nanotubes, which are 16 nanometers in diameter and several micrometers long, a molecular layer of electron-accepting trinitrofluorenone laminates an electron-donating graphitic layer of π-stacked hexabenzocoronene. The coaxial nanotubular structure allows photochemical generation of spatially separated charge carriers and a quick photoconductive response with a large on/off ratio greater than 10 4 . In sharp contrast, the microfibers consist of a charge-transfer complex between the hexabenzocoronene and trinitrofluorenone parts and exhibit almost no photocurrent generation.
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Citations
Cited by
Yashima, E., Ousaka, N., Taura, D., Shimomura, K., Ikai, T., & Maeda, K. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00354 · Cited by 2,004
Challenges and breakthroughs in recent research on self-assembly
Ariga, K., Hill, J. P., Lee, M. V., Vinu, A., Charvet, R., & Acharya, S. (2008) · Science and Technology of Advanced Materials · doi:10.1088/1468-6996/9/1/014109 · Cited by 759
Discotic Liquid Crystals for Opto-Electronic Applications
Kaafarani, B. R. (2011) · Chemistry of Materials · doi:10.1021/cm102117c · Cited by 513
Supramolecular Chemistry and Self-Assembly in Organic Materials Design
Stupp, S. I., & Palmer, L. C. (2014) · Chemistry of Materials · doi:10.1021/cm403028b · Cited by 513
Emerging tellurium nanostructures: controllable synthesis and their applications
He, Z., Yang, Y., Liu, J.-W., & Yu, S.-H. (2017) · Chemical Society Reviews · doi:10.1039/c7cs00013h · Cited by 282
Metadata
- Authors
- Yamamoto, Y., Fukushima, T., Suna, Y., Ishii, N., Saeki, A., Seki, S., Tagawa, S., Taniguchi, M., Kawai, T., & Aida, T.
- Venue
- Science
- Published
- 2006-12-15
- Volume
- 314
- Issue
- 5806
- Pages
- 1761-1764
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2001187576
- Cited by
- 705
- References
- 0
- FWCI
- 27.58
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yamamoto, Y., Fukushima, T., Suna, Y., Ishii, N., Saeki, A., Seki, S., Tagawa, S., Taniguchi, M., Kawai, T., & Aida, T. (2006). Photoconductive Coaxial Nanotubes of Molecularly Connected Electron Donor and Acceptor Layers. Science. https://doi.org/10.1126/science.1134441
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