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Electronic Structure Controls Reactivity of Size-Selected Pd Clusters Adsorbed on TiO 2 Surfaces
Abstract
Cluster Electronics and Catalysis: Many practical catalysts consist of small metal clusters on oxide supports, and the activity of these clusters usually varies with their size. In order to sort out some of the competing effects that lead to such variations, Kaden et al. (p. 826 ) size-selected palladium clusters (from single atoms to clusters up to 25 atoms) and deposited them on a crystal face of the rutile phase of titanium dioxide. X-ray photoemission studies and temperature-programmed reaction measurements showed that the activity of these model catalysts for CO oxidation was related to the electronic energy, which was reflected in the Pd 3d electron binding energy. Ion-scattering studies showed that the clusters formed flat single- or double-layer islands.
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Citations
Cites
Identification of Active Gold Nanoclusters on Iron Oxide Supports for CO Oxidation
Herzing, A. A., Kiely, C. J., Carley, A. F., Landon, P., & Hutchings, G. J. (2008) · Science · doi:10.1126/science.1159639 · Cited by 1,530
Cited by
Single-atom catalysis of CO oxidation using Pt1/FeOx
Qiao, B., Wang, A., Yang, X., Allard, L. F., Jiang, Z., Cui, Y., Liu, J., Li, J., & Zhang, T. (2011) · Nature Chemistry · doi:10.1038/nchem.1095 · Cited by 7,526
Catalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Titanium Dioxide Crystals with Tailored Facets
Liu, G., Yang, H. G., Pan, J., Yang, Y. Q., Lu, G. Q. (., & Cheng, H.-M. (2014) · Chemical Reviews · doi:10.1021/cr400621z · Cited by 1,084
The Power of Single‐Atom Catalysis
Liang, S., Hao, C., & Shi, Y. (2015) · ChemCatChem · doi:10.1002/cctc.201500363 · Cited by 365
Recent advances in the precise control of isolated single-site catalysts by chemical methods
Li, Z., Wang, D., Wu, Y., & Li, Y. (2018) · National Science Review · doi:10.1093/nsr/nwy056 · Cited by 325
Metadata
- Authors
- Kaden, W. E., Wu, T., Kunkel, W. A., & Anderson, S. L.
- Venue
- Science
- Published
- 2009-11-06
- Volume
- 326
- Issue
- 5954
- Pages
- 826-829
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2033270806
- Cited by
- 633
- References
- 1
- FWCI
- 13.08
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kaden, W. E., Wu, T., Kunkel, W. A., & Anderson, S. L. (2009). Electronic Structure Controls Reactivity of Size-Selected Pd Clusters Adsorbed on TiO 2 Surfaces. Science. https://doi.org/10.1126/science.1180297
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
