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Spontaneous and X-ray–Triggered Crystallization at Long Range in Self-Assembling Filament Networks
Open accessAbstract
X-rays to Order: Self-assembly of molecules is often irreversible. Cui et al. (p. 555 , published online 17 December; see the Perspective by Safinya and Li ) examined the ordering of a short peptide sequence (Ala 6 Glu 3 ) terminated with an alkyl chain. Aqueous solutions of this molecule could form hexagonally ordered filaments, but more dilute solutions were disordered. However, prolonged x-ray exposure caused these arrays to become ordered. These arrays were stable for several hours but eventually returned to a disordered state; the addition of salts slowed the ordering processes. It is possible that during the ordering process, X-ray–induced charging affected the repulsive forces that balance tension within the filament.
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Cited by
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Supramolecular Chemistry and Self-Assembly in Organic Materials Design
Stupp, S. I., & Palmer, L. C. (2014) · Chemistry of Materials · doi:10.1021/cm403028b · Cited by 513
Self-citationCheetham, A. G., Chakroun, R. W., Ma, W., & Cui, H. (2017) · Chem. Soc. Rev. · doi:10.1039/c7cs00521k · Cited by 367
Self-citationNewcomb, C. J., Moyer, T. J., Lee, S. S., & Stupp, S. I. (2012) · Current Opinion in Colloid & Interface Science · doi:10.1016/j.cocis.2012.09.004 · Cited by 76
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Metadata
- Authors
- Cui, H., Pashuck, E. T., Velichko, Y. S., Weigand, S. J., Cheetham, A. G., Newcomb, C. J., & Stupp, S. I.
- Venue
- Science
- Published
- 2010-01-29
- Volume
- 327
- Issue
- 5965
- Pages
- 555-559
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2062194766
- Cited by
- 172
- References
- 0
- FWCI
- 5.74
- Type
- journal article
- Language
- en
- Open access
- green
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- Cui, H., Pashuck, E. T., Velichko, Y. S., Weigand, S. J., Cheetham, A. G., Newcomb, C. J., & Stupp, S. I. (2010). Spontaneous and X-ray–Triggered Crystallization at Long Range in Self-Assembling Filament Networks. Science. https://doi.org/10.1126/science.1182340
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