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Direct Imaging of Covalent Bond Structure in Single-Molecule Chemical Reactions
Abstract
Watching Organic Reactions: Single-molecule studies can overcome the difficulty of inferring the various outcomes of reactions in ensemble measurements. De Oteyza et al. (p. 1434 , published online 30 May; see the Perspective by Giessibl ) used a variation of noncontact atomic force microscopy in which the imaging tip was derivatized with a single CO molecule to obtain subnanometer-resolution images of conjugated organic molecules undergoing reaction on a silver surface. Different thermally induced cyclization reactions of oligo- (phenylene-1,2-ethynylenes) were observed.
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Cites
Self-interaction correction to density-functional approximations for many-electron systems
Perdew, J. P., & Zunger, A. (1981) · Physical Review B · doi:10.1103/physrevb.23.5048 · Cited by 20,887
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Metadata
- Authors
- de Oteyza, D. G., Gorman, P., Chen, Y.-C., Wickenburg, S., Riss, A., Mowbray, D. J., Etkin, G., Pedramrazi, Z., Tsai, H.-Z., Rubio, A., Crommie, M. F., & Fischer, F. R.
- Venue
- Science
- Published
- 2013-06-21
- Volume
- 340
- Issue
- 6139
- Pages
- 1434-1437
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1969699263
- Cited by
- 632
- References
- 1
- FWCI
- 30.47
- Type
- journal article
- Language
- en
- Open access
- closed
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- de Oteyza, D. G., Gorman, P., Chen, Y.-C., Wickenburg, S., Riss, A., Mowbray, D. J., Etkin, G., Pedramrazi, Z., Tsai, H.-Z., Rubio, A., Crommie, M. F., & Fischer, F. R. (2013). Direct Imaging of Covalent Bond Structure in Single-Molecule Chemical Reactions. Science. https://doi.org/10.1126/science.1238187
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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