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Ground Water Redox Reactions: An Analysis of Equilibrium State Applied to Eh Measurements and Geochemical Modeling
Abstract
Computer modeling of 611 high-quality analyses of normal ground waters from diverse geographic areas reveals that aqueous oxidation-reduction reactions are generally not at equilibrium. Multiple redox couples present in individual samples yield computed Nernstian Eh (redox potential) values spanning as much as 1000 millivolts. The computed Eh values do not agree with each other, nor do they agree with the single "master" value measured in the field with a platinum electrode. Because of internal disequilibrium, the use of any measured Eh value as input to equilibrium hydrogeochemical computer models will generally yield misleading results for normal ground waters.
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Cited by
A review of the source, behaviour and distribution of arsenic in natural waters
Smedley, P. L., & Kinniburgh, D. G. (2002) · Applied Geochemistry · doi:10.1016/s0883-2927(02)00018-5 · Cited by 7,691
Arsenic in Ground Water of the United States: Occurrence and Geochemistry
Welch, A. H., Westjohn, D. B., Helsel, D. R., & Wanty, R. B. (2000) · Groundwater · doi:10.1111/j.1745-6584.2000.tb00251.x · Cited by 893
Sasaki, T., Watanabe, M., Hashizume, H., Yamada, H., & Nakazawa, H. (1996) · Journal of the American Chemical Society · doi:10.1021/ja960073b · Cited by 869
Redoxable Nanosheet Crystallites of MnO2 Derived via Delamination of a Layered Manganese Oxide
Omomo, Y., Sasaki, T., Wang, & Watanabe, M. (2003) · Journal of the American Chemical Society · doi:10.1021/ja021364p · Cited by 718
Lovley, D. R., & Goodwin, S. (1988) · Geochimica et Cosmochimica Acta · doi:10.1016/0016-7037(88)90163-9 · Cited by 659
Metadata
- Authors
- Lindberg, R. D., & Runnells, D. D.
- Venue
- Science
- Published
- 1984-08-31
- Volume
- 225
- Issue
- 4665
- Pages
- 925-927
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1976119057
- Cited by
- 433
- References
- 0
- FWCI
- 16.60
- Type
- journal article
- Language
- en
- Open access
- closed
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- Lindberg, R. D., & Runnells, D. D. (1984). Ground Water Redox Reactions: An Analysis of Equilibrium State Applied to Eh Measurements and Geochemical Modeling. Science. https://doi.org/10.1126/science.225.4665.925
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