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Effect of Substrate Strain on Adsorption
Abstract
Direct evidence for the effect of local strain at a surface on the bonding strength for adsorbates is presented. Scanning tunneling microscopy revealed that adsorbed oxygen atoms on Ru(0001) surfaces are located preferentially on top of nanometer-size protrusions above subsurface argon bubbles, where tensile strain prevails, and are depleted around their rim in regions of compression, relative to the flat surface. Such effects can be considered as the reverse of adsorbate-induced strain, and their direct local demonstration can be used to test theoretical predictions.
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Cited by
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Diebold, U. (2003) · Surface Science Reports · doi:10.1016/s0167-5729(02)00100-0 · Cited by 7,944
Progress and perspectives of electrochemical CO2 reduction on copper in aqueous electrolyte
Nitopi, S., Bertheussen, E., Scott, S. B., Liu, X., Engstfeld, A. K., Horch, S., Seger, B., Stephens, I. E. L., Chan, K., Hahn, C., et al. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00705 · Cited by 5,223
Theoretical surface science and catalysis—calculations and concepts
Hammer, B., & Nørskov, J. K. (2000) · Advances in Catalysis · doi:10.1016/s0360-0564(02)45013-4 · Cited by 3,972
Effect of Strain on the Reactivity of Metal Surfaces
Mavrikakis, M., Hammer, B., & Nørskov, J. K. (1998) · Physical Review Letters · doi:10.1103/physrevlett.81.2819 · Cited by 2,380
Strain-controlled electrocatalysis on multimetallic nanomaterials
Luo, M., & Guo, S. (2017) · Nature Reviews Materials · doi:10.1038/natrevmats.2017.59 · Cited by 1,115
Metadata
- Authors
- Gsell, M., Jakob, P., & Menzel, D.
- Venue
- Science
- Published
- 1998-05
- Volume
- 280
- Issue
- 5364
- Pages
- 717-720
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2150234030
- Cited by
- 394
- References
- 0
- FWCI
- 8.59
- Type
- journal article
- Language
- en
- Open access
- closed
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- Gsell, M., Jakob, P., & Menzel, D. (1998). Effect of Substrate Strain on Adsorption. Science. https://doi.org/10.1126/science.280.5364.717
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