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Carbon Structures with Three-Dimensional Periodicity at Optical Wavelengths
Abstract
Porous carbons that are three-dimensionally periodic on the scale of optical wavelengths were made by a synthesis route resembling the geological formation of natural opal. Porous silica opal crystals were sintered to form an intersphere interface through which the silica was removed after infiltration with carbon or a carbon precursor. The resulting porous carbons had different structures depending on synthesis conditions. Both diamond and glassy carbon inverse opals resulted from volume filling. Graphite inverse opals, comprising 40-angstrom-thick layers of graphite sheets tiled on spherical surfaces, were produced by surface templating. The carbon inverse opals provide examples of both dielectric and metallic optical photonic crystals. They strongly diffract light and may provide a route toward photonic band-gap materials.
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Citations
Cited by
Mesoporous carbon materials: Synthesis and modification
Liang, C., Li, Z., & Dai, S. (2008) · Angewandte Chemie International Edition · doi:10.1002/anie.200702046 · Cited by 1,935
Yin, Y., Lu, Y., Gates, B., & Xia, Y. (2001) · Journal of the American Chemical Society · doi:10.1021/ja011048v · Cited by 915
Synthesis of a large-scale highly ordered porous carbon film by self-assembly of block copolymers
Liang, C., Hong, K., Guiochon, G. A., Mays, J. W., & Dai, S. (2004) · Angewandte Chemie International Edition · doi:10.1002/anie.200461051 · Cited by 834
Synthesis of a new mesoporous carbon and its application to electrochemical double-layer capacitors
Lee, J., Yoon, S., Hyeon, T., Oh, S. M., & Kim, K. B. (1999) · Chemical Communications · doi:10.1039/a906872d · Cited by 774
Templated nanocarbons for energy storage
Nishihara, H., & Kyotani, T. (2012) · Advanced Materials · doi:10.1002/adma.201201715 · Cited by 745
Metadata
- Authors
- Zakhidov, A. A., Baughman, R. H., Iqbal, Z., Cui, C., Khayrullin, I., Dantas, S. O., Marti, J., & Ralchenko, V. G.
- Venue
- Science
- Published
- 1998-10-30
- Volume
- 282
- Issue
- 5390
- Pages
- 897-901
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2140133212
- Cited by
- 1,067
- References
- 0
- FWCI
- 39.99
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zakhidov, A. A., Baughman, R. H., Iqbal, Z., Cui, C., Khayrullin, I., Dantas, S. O., Marti, J., & Ralchenko, V. G. (1998). Carbon Structures with Three-Dimensional Periodicity at Optical Wavelengths. Science. https://doi.org/10.1126/science.282.5390.897
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