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Self-Assembly of Ordered Microporous Materials from Rod-Coil Block Copolymers
Abstract
Rod-coil diblock copolymers in a selective solvent for the coil-like polymer self-organize into hollow spherical micelles having diameters of a few micrometers. Long-range, close-packed self-ordering of the micelles produced highly iridescent periodic microporous materials. Solution-cast micellar films consisted of multilayers of hexagonally ordered arrays of spherical holes whose diameter, periodicity, and wall thickness depended on copolymer molecular weight and composition. Addition of fullerenes into the copolymer solutions also regulated the microstructure and optical properties of the microporous films. These results demonstrate the potential of hierarchical self-assembly of macromolecular components for engineering complex two- and three-dimensional periodic and functional mesostructures.
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Zhang, L., & Eisenberg, A. (1996) · Journal of the American Chemical Society · doi:10.1021/ja953709s · Cited by 1,262
Cited by
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Bioinspired engineering of honeycomb structure – Using nature to inspire human innovation
Zhang, Q., Yang, X., Li, P., Huang, G., Feng, S., Shen, C., Han, B., Zhang, X., Jin, F., Xu, F., et al. (2015) · Progress in Materials Science · doi:10.1016/j.pmatsci.2015.05.001 · Cited by 836
Nanostructure fabrication using block copolymers
Hamley, I. W. (2003) · Nanotechnology · doi:10.1088/0957-4484/14/10/201 · Cited by 773
Catalyst layer ink interactions that affect coatability
Dixit, M. B., Harkey, B. A., Shen, F., & Hatzell, K. B. (2018) · Journal of The Electrochemical Society · doi:10.1149/2.0191805jes · Cited by 126
Micellar Morphological Changes Promoted by Cyclization of PS-b-PI Copolymer: DLS and AFM Experiments
Minatti, E., Viville, P., Borsali, R., Schappacher, M., Deffieux, A., & Lazzaroni, R. (2003) · Macromolecules · doi:10.1021/ma020927e · Cited by 98
Metadata
- Authors
- Jenekhe, S. A., & Chen, X. L.
- Venue
- Science
- Published
- 1999-01-15
- Volume
- 283
- Issue
- 5400
- Pages
- 372-375
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1966608618
- Cited by
- 929
- References
- 1
- FWCI
- 31.45
- Type
- journal article
- Language
- en
- Open access
- closed
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- Jenekhe, S. A., & Chen, X. L. (1999). Self-Assembly of Ordered Microporous Materials from Rod-Coil Block Copolymers. Science. https://doi.org/10.1126/science.283.5400.372
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
