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Green, Catalytic Oxidation of Alcohols in Water
Abstract
Alcohol oxidations are typically performed with stoichiometric reagents that generate heavy-metal waste and are usually run in chlorinated solvents. A water-soluble palladium(II) bathophenanthroline complex is a stable recyclable catalyst for the selective aerobic oxidation of a wide range of alcohols to aldehydes, ketones, and carboxylic acids in a biphasic water-alcohol system. The use of water as a solvent and air as the oxidant makes the reaction interesting from both an economic and environmental point of view.
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Citations
Cited by
Solvent-Free Oxidation of Primary Alcohols to Aldehydes Using Au-Pd/TiO 2 Catalysts
Enache, D. I., Edwards, J. K., Landon, P., Solsona-Espriu, B., Carley, A. F., Herzing, A. A., Watanabe, M., Kiely, C. J., Knight, D. W., & Hutchings, G. J. (2006) · Science · doi:10.1126/science.1120560 · Cited by 2,106
Supported gold nanoparticles as catalysts for organic reactions
Corma, A., & Garcia, H. (2008) · Chemical Society Reviews · doi:10.1039/b707314n · Cited by 1,883
Green oxidation with aqueous hydrogen peroxide
Noyori, R., Aoki, M., & Sato, K. (2003) · Chemical Communications · doi:10.1039/b303160h · Cited by 1,085
Mori, K., Hara, T., Mizugaki, T., Ebitani, K., & Kaneda, K. (2004) · Journal of the American Chemical Society · doi:10.1021/ja0488683 · Cited by 939
Metadata
- Authors
- Brink, G.-J. T., Arends, I. W. C. E., & Sheldon, R. A.
- Venue
- Science
- Published
- 2000-03-03
- Volume
- 287
- Issue
- 5458
- Pages
- 1636-1639
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2144828032
- Cited by
- 1,156
- References
- 0
- FWCI
- 31.66
- Type
- journal article
- Language
- en
- Open access
- closed
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- Brink, G.-J. T., Arends, I. W. C. E., & Sheldon, R. A. (2000). Green, Catalytic Oxidation of Alcohols in Water. Science. https://doi.org/10.1126/science.287.5458.1636
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Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
