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Quantized Phonon Spectrum of Single-Wall Carbon Nanotubes
Open accessAbstract
The electronic spectra of carbon nanotubes and other nanoscale systems are quantized because of their small radii. Similar quantization in the phonon spectra has been difficult to observe because of the far smaller energy scale. We probed this regime by measuring the temperature-dependent specific heat of purified single-wall nanotubes. The data show direct evidence of one-dimensional quantized phonon subbands. Above 4 kelvin, they are in excellent agreement with model calculations of individual nanotubes and differ markedly from the specific heat of two-dimensional graphene or three-dimensional graphite. Detailed modeling yields an energy of 4.3 millielectron volts for the lowest quantized phonon subband and a tube-tube (or “lattice”) Debye energy of 1.1 millielectron volts, implying a small intertube coupling in bundles.
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Cites
High-field electrical transport in single-wall carbon nanotubes
Yao, Z., Kane, C. L., & Dekker, C. (2000) · Physical Review Letters · doi:10.1103/physrevlett.84.2941 · Cited by 1,501
Cited by
Thermal Transport Measurements of Individual Multiwalled Nanotubes
Kim, P., Shi, L., Majumdar, A., & McEuen, P. L. (2001) · Physical Review Letters · doi:10.1103/physrevlett.87.215502 · Cited by 3,378
Superhydrophobic Carbon Nanotube Forests
Lau, K. K. S., Bico, J., Teo, K. B. K., Chhowalla, M., Amaratunga, G. A. J., Milne, W. I., McKinley, G. H., & Gleason, K. K. (2003) · Nano Letters · doi:10.1021/nl034704t · Cited by 1,537
Interfacial Heat Flow in Carbon Nanotube Suspensions
Huxtable, S. T., Cahill, D. G., Shenogin, S., Xue, L., Ozisik, R., Barone, P., Usrey, M., Strano, M. S., Siddons, G., Shim, M., et al. (2003) · Nature Materials · doi:10.1038/nmat996 · Cited by 1,023
Carbon Nanotube−Inorganic Hybrids
Eder, D. (2010) · Chemical Reviews · doi:10.1021/cr800433k · Cited by 819
Qiu, L., Zhu, N., Feng, Y., Michaelides, E. E., Żyła, G., Jing, D., Zhang, X., Norris, P. M., Markides, C. N., & Mahian, O. (2020) · Physics Reports · doi:10.1016/j.physrep.2019.12.001 · Cited by 523
Metadata
- Authors
- Hone, J., Batlogg, B., Benes, Z., Johnson, A. T., & Fischer, J. E.
- Venue
- Science
- Published
- 2000-09-08
- Volume
- 289
- Issue
- 5485
- Pages
- 1730-1733
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2046305345
- Cited by
- 506
- References
- 1
- FWCI
- 15.01
- Type
- journal article
- Language
- en
- Open access
- green
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- Hone, J., Batlogg, B., Benes, Z., Johnson, A. T., & Fischer, J. E. (2000). Quantized Phonon Spectrum of Single-Wall Carbon Nanotubes. Science. https://doi.org/10.1126/science.289.5485.1730
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