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A rational strategy for the realization of chain-growth supramolecular polymerization
Abstract
Popping open one by one into polymers: We rarely board airplanes by joining the back of a single well-ordered line. More often, we jostle around in one of several bulging crowds that merge haphazardly near the gate. Roughly speaking, these processes are analogous to the chain growth and step growth mechanisms of polymer assembly at the molecular level. Kang et al. present a strategy to link molecular building blocks through hydrogen bonding in accord with the well-controlled chain growth model. The molecules start out curled inward, as they engage in internal hydrogen bonding, until an initiator pulls one open; that molecule is then in the right conformation to pull a partner into the growing chain, poising it to pull in yet another, and so forth down the line. Science , this issue p. 646
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Odian, G. (2004) · doi:10.1002/047147875x · Cited by 7,158
Stereoselective Epoxide Polymerization and Copolymerization
Childers, M. I., Longo, J. M., Van Zee, N. J., LaPointe, A. M., & Coates, G. W. (2014) · Chemical Reviews · doi:10.1021/cr400725x · Cited by 471
Cited by
Yashima, E., Ousaka, N., Taura, D., Shimomura, K., Ikai, T., & Maeda, K. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00354 · Cited by 2,004
Non-equilibrium supramolecular polymerization
Sorrenti, A., Leira-Iglesias, J., Markvoort, A. J., de Greef, T. F. A., & Hermans, T. M. (2017) · Chemical Society Reviews · doi:10.1039/c7cs00121e · Cited by 574
Control over differentiation of a metastable supramolecular assembly in one and two dimensions
Fukui, T., Kawai, S., Fujinuma, S., Matsushita, Y., Yasuda, T., Sakurai, T., Seki, S., Takeuchi, M., & Sugiyasu, K. (2017) · Nature Chemistry · doi:10.1038/nchem.2684 · Cited by 554
Interfacial Polymerization: From Chemistry to Functional Materials
Zhang, F., Fan, J., & Wang, S. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201916473 · Cited by 478
50th Anniversary Perspective: Living Polymerization—Emphasizing the Molecule in Macromolecules
Grubbs, R. B., & Grubbs, R. H. (2017) · Macromolecules · doi:10.1021/acs.macromol.7b01440 · Cited by 396
Metadata
- Authors
- Kang, J., Miyajima, D., Mori, T., Inoue, Y., Itoh, Y., & Aida, T.
- Venue
- Science
- Published
- 2015-02-06
- Volume
- 347
- Issue
- 6222
- Pages
- 646-651
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2027685213
- Cited by
- 665
- References
- 2
- FWCI
- 29.22
- Type
- journal article
- Language
- en
- Open access
- closed
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- Kang, J., Miyajima, D., Mori, T., Inoue, Y., Itoh, Y., & Aida, T. (2015). A rational strategy for the realization of chain-growth supramolecular polymerization. Science. https://doi.org/10.1126/science.aaa4249
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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