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Identification of active sites in CO oxidation and water-gas shift over supported Pt catalysts
Abstract
Comparing active site reactivity: Noble metal nanoparticles often exhibit behaviors distinct from atomic and bulk versions of the same material. Gold and platinum dispersed on metal oxide supports, for example, show remarkable low-temperature reactivity for carbon monoxide (CO) oxidation by oxygen or water. Ding et al. used infrared spectroscopy to identify CO adsorbed on isolated platinum atoms or nanoparticles dispersed on zeolite and oxide supports. Temperature-programmed desorption studies showed that CO reacted at much lower temperatures when adsorbed on nanoparticles versus on isolated metal atoms. Science , this issue p. 189
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Cites
Identification of Active Gold Nanoclusters on Iron Oxide Supports for CO Oxidation
Herzing, A. A., Kiely, C. J., Carley, A. F., Landon, P., & Hutchings, G. J. (2008) · Science · doi:10.1126/science.1159639 · Cited by 1,530
Cited by
Catalysis by Supported Single Metal Atoms
Liu, J. (2017) · ACS Catalysis · doi:10.1021/acscatal.6b01534 · Cited by 1,331
Heterogeneous Single-Atom Photocatalysts: Fundamentals and Applications
Gao, C., Low, J., Long, R., Kong, T., Zhu, J., & Xiong, Y. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00840 · Cited by 1,050
Cao, L., Luo, Q., Liu, W., Lin, Y., Liu, X., Cao, Y., Zhang, W., Wu, Y., Yang, J., Yao, T., et al. (2018) · Nature Catalysis · doi:10.1038/s41929-018-0203-5 · Cited by 901
Tuning selectivity of electrochemical reactions by atomically dispersed platinum catalyst
Choi, C. H., Kim, M., Kwon, H. C., Cho, S. J., Yun, S., Kim, H.-T., Mayrhofer, K. J. J., Kim, H., & Choi, M. (2016) · Nature Communications · doi:10.1038/ncomms10922 · Cited by 849
Single Pt Atoms Confined into a Metal–Organic Framework for Efficient Photocatalysis
Fang, X., Shang, Q., Wang, Y., Jiao, L., Yao, T., Li, Y., Zhang, Q., Luo, Y., & Jiang, H. (2018) · Advanced Materials · doi:10.1002/adma.201705112 · Cited by 837
Metadata
- Authors
- Ding, K., Gulec, A., Johnson, A. M., Schweitzer, N. M., Stucky, G. D., Marks, L. D., & Stair, P. C.
- Venue
- Science
- Published
- 2015-10-09
- Volume
- 350
- Issue
- 6257
- Pages
- 189-192
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W1853374276
- Cited by
- 1,272
- References
- 1
- FWCI
- 26.65
- Type
- journal article
- Language
- en
- Open access
- closed
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- Ding, K., Gulec, A., Johnson, A. M., Schweitzer, N. M., Stucky, G. D., Marks, L. D., & Stair, P. C. (2015). Identification of active sites in CO oxidation and water-gas shift over supported Pt catalysts. Science. https://doi.org/10.1126/science.aac6368
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