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Photosensitized, energy transfer-mediated organometallic catalysis through electronically excited nickel(II)
Open accessAbstract
A nickel's worth of transferred energy: Traditional organic photochemistry often relies on sensitizers, molecules that efficiently absorb light and then transfer the energy to other compounds to spur reactivity. Welin et al. leveraged this approach to stimulate an organometallic nickel catalyst. They photoexcited an iridium complex with blue light. The ensuing energy transfer to nickel enabled C–O bond formation, coupling aryl halides with carboxylic acids. A similar approach could generate a variety of additional reactivity patterns through photosensitized transition metal catalysis. Science , this issue p. 380
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Cited by
Triplet Energy Transfer Photocatalysis: Unlocking the Next Level
Strieth-Kalthoff, F., & Glorius, F. (2020) · Chem · doi:10.1016/j.chempr.2020.07.010 · Cited by 650
Tay, N. E. S., Lehnherr, D., & Rovis, T. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00384 · Cited by 518
Irradiation-Induced Heck Reaction of Unactivated Alkyl Halides at Room Temperature
Wang, G.-Z., Shang, R., Cheng, W.-M., & Fu, Y. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.7b10009 · Cited by 341
Zhu, C., Yue, H., Jia, J., & Rueping, M. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202013852 · Cited by 259
Chasing the rainbow: Exploiting photosensitizers to drive photoisomerization reactions
Wang, Z., Fernandez, L., Aslam, A. S., Shamsabadi, M., Muhammad, L. M., & Moth‐Poulsen, K. (2023) · Responsive Materials · doi:10.1002/rpm.20230012 · Cited by 28
Metadata
- Authors
- Welin, E. R., Le, C., Arias-Rotondo, D. M., McCusker, J. K., & MacMillan, D. W. C.
- Venue
- Science
- Published
- 2017-01-27
- Volume
- 355
- Issue
- 6323
- Pages
- 380-385
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W2580635944
- Cited by
- 558
- References
- 0
- FWCI
- 23.00
- Type
- journal article
- Language
- en
- Open access
- green
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- Welin, E. R., Le, C., Arias-Rotondo, D. M., McCusker, J. K., & MacMillan, D. W. C. (2017). Photosensitized, energy transfer-mediated organometallic catalysis through electronically excited nickel(II). Science. https://doi.org/10.1126/science.aal2490
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
