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Conformal quantum dot–SnO 2 layers as electron transporters for efficient perovskite solar cells
Open accessAbstract
Improvements to perovskite solar cells (PSCs) have focused on increasing their power conversion efficiency (PCE) and operational stability and maintaining high performance upon scale-up to module sizes. We report that replacing the commonly used mesoporous–titanium dioxide electron transport layer (ETL) with a thin layer of polyacrylic acid–stabilized tin(IV) oxide quantum dots (paa-QD-SnO 2 ) on the compact–titanium dioxide enhanced light capture and largely suppressed nonradiative recombination at the ETL–perovskite interface. The use of paa-QD-SnO 2 as electron-selective contact enabled PSCs (0.08 square centimeters) with a PCE of 25.7% (certified 25.4%) and high operational stability and facilitated the scale-up of the PSCs to larger areas. PCEs of 23.3, 21.7, and 20.6% were achieved for PSCs with active areas of 1, 20, and 64 square centimeters, respectively.
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Cites
Efficient perovskite solar cells via improved carrier management
Yoo, J. J., Seo, G., Chua, M. R., Park, T. G., Lu, Y., Rotermund, F., Kim, Y.-K., Moon, C. S., Jeon, N. J., Correa-Baena, J.-P., et al. (2021) · Nature · doi:10.1038/s41586-021-03285-w · Cited by 2,934
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Cited by
Unveiling facet-dependent degradation and facet engineering for stable perovskite solar cells
Ma, C., Eickemeyer, F. T., Lee, S.-H., Kang, D.-H., Kwon, S. J., Grätzel, M., & Park, N.-G. (2023) · Science · doi:10.1126/science.adf3349 · Cited by 423
Self-citationZheng, X., Li, Z., Zhang, Y., Chen, M., Liu, T., Xiao, C., Gao, D., Patel, J. B., Kuciauskas, D., Magomedov, A., et al. (2023) · Nature Energy · doi:10.1038/s41560-023-01227-6 · Cited by 359
Zhou, Y., Herz, L. M., Jen, A. K.-Y., & Saliba, M. (2022) · Nature Energy · doi:10.1038/s41560-022-01096-5 · Cited by 281
Operationally stable perovskite solar modules enabled by vapor-phase fluoride treatment
Zhao, X., Zhang, P., Liu, T., Tian, B., Jiang, Y., Zhang, J., Tang, Y., Li, B., Xue, M., Zhang, W., et al. (2024) · Science · doi:10.1126/science.adn9453 · Cited by 152
Recent progress in perovskite solar cells: from device to commercialization
Luo, X., Lin, X., Gao, F., Zhao, Y., Li, X., Zhan, L., Qiu, Z., Wang, J., Chen, C., Meng, L., et al. (2022) · Science China Chemistry · doi:10.1007/s11426-022-1426-x · Cited by 142
Metadata
- Authors
- Kim, M., Jeong, J., Lu, H., Lee, T. K., Eickemeyer, F. T., Liu, Y., Choi, I. W., Choi, S. J., Jo, Y., Kim, H.-B., Mo, S.-I., Kim, Y.-K., Lee, H., An, N. G., Cho, S., Tress, W. R., Zakeeruddin, S. M., Hagfeldt, A., Kim, J. Y., Grätzel, M., & Kim, D. S.
- Venue
- Science
- Published
- 2022-01-21
- Volume
- 375
- Issue
- 6578
- Pages
- 302-306
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W4206188804
- Cited by
- 1,346
- References
- 1
- FWCI
- 84.18
- Type
- journal article
- Language
- en
- Open access
- green
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- Kim, M., Jeong, J., Lu, H., Lee, T. K., Eickemeyer, F. T., Liu, Y., Choi, I. W., Choi, S. J., Jo, Y., Kim, H.-B., Mo, S.-I., Kim, Y.-K., Lee, H., An, N. G., Cho, S., Tress, W. R., Zakeeruddin, S. M., Hagfeldt, A., Kim, J. Y., . . . Kim, D. S. (2022). Conformal quantum dot–SnO 2 layers as electron transporters for efficient perovskite solar cells. Science. https://doi.org/10.1126/science.abh1885
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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