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Sabatier principle of metal-support interaction for design of ultrastable metal nanocatalysts
Abstract
Rational design of stable nanocatalysts: Sintering of nanoparticles is one of the main causes of their catalytic deactivation. Rational design of nanocatalysts that are stable against sintering is a grand challenge in heterogenous catalysis. Hu et al . present kinetic theories for two competing sintering mechanisms, Ostwald ripening and particle migration, which relate the rates of both processes to fundamental interaction energies in metal nanoparticle-support combinations. Using kinetic simulations for hundreds of such pairs, the authors show a universal volcano dependence of the sintering kinetics on the metal-support binding energy that can serve as a single descriptor to predict nanoparticle growth rates. The revealed scaling relations are a good start in the development of high-throughput screening computational approaches to drive discovery of sintering-resistant nanocatalysts. —YS
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Generalized Gradient Approximation Made Simple
Perdew, J. P., Burke, K., & Ernzerhof, M. (1996) · Physical Review Letters · doi:10.1103/physrevlett.77.3865 · Cited by 215,824
Efficient iterative schemes for ab initio total-energy calculations using a plane-wave basis set
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Cited by
Recent progress on the long‐term stability of hydrogen evolution reaction electrocatalysts
Zhai, W., Ma, Y., Chen, D., Ho, J. C., Dai, Z., & Qu, Y. (2022) · InfoMat · doi:10.1002/inf2.12357 · Cited by 375
Spin-dependent electrocatalysis
Chen, Z., Li, X., Ma, H., Zhang, Y., Peng, J., Ma, T., Cheng, Z., Gracia, J., Sun, Y., & Xu, Z. J. (2024) · National Science Review · doi:10.1093/nsr/nwae314 · Cited by 100
Yu, S., & Yang, H. (2023) · Chemical Communications · doi:10.1039/d3cc00590a · Cited by 33
Metadata
- Authors
- Hu, S., & Li, W.-X.
- Venue
- Science
- Published
- 2021-12-10
- Volume
- 374
- Issue
- 6573
- Pages
- 1360-1365
- ISSN
- 0036-8075 (ISSN-L)
- 1095-9203
- OpenAlex
- W3210780992
- Cited by
- 821
- References
- 2
- FWCI
- 30.23
- Type
- journal article
- Language
- en
- Open access
- closed
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