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Cited by 205

The DOI matches its Crossref record; 7 of the 7 references it cites were found in a registry or an index.

Truly combining the advantages of polymeric and zeolite membranes for gas separations

Open access
Tan, Xiaoyu, Robijns, Sven, Thür, Raymond, Ke, Quanli, De Witte, Niels, Lamaire, Aran, Li, Yun, Aslam, Imran, Van Havere, Daan, Donckels, Thibaut, Van Assche, Tom, Van Speybroeck, Veronique, Dusselier, Michiel, Vankelecom, Ivo·2022·Science

Abstract

Mixed-matrix membranes (MMMs) have been investigated to render energy-intensive separations more efficiently by combining the selectivity and permeability performance, robustness, and nonaging properties of the filler with the easy processing, handling, and scaling up of the polymer. However, truly combining all in one single material has proven very challenging. In this work, we filled a commercial polyimide with ultrahigh loadings of a high–aspect ratio, CO 2 -philic Na-SSZ-39 zeolite with a three-dimensional channel system that precisely separates gas molecules. By carefully designing both zeolite and MMM synthesis, we created a gas-percolation highway across a flexible and aging-resistant (more than 1 year) membrane. The combination of a CO 2 -CH 4 mixed-gas selectivity of ~423 and a CO 2 permeability of ~8300 Barrer outperformed all existing polymer-based membranes and even most zeolite-only membranes.

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Registry

Crossref · 10.1126/science.ade1411

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Metadata

Authors
Tan, X., Robijns, S., Thür, R., Ke, Q., De Witte, N., Lamaire, A., Li, Y., Aslam, I., Van Havere, D., Donckels, T., Van Assche, T., Van Speybroeck, V., Dusselier, M., & Vankelecom, I.
Venue
Science
Published
2022-12-16
Volume
378
Issue
6625
Pages
1189-1194
ISSN
  • 0036-8075 (ISSN-L)
  • 1095-9203
OpenAlex
W4311551606
Cited by
205
References
7
FWCI
14.58
Type
journal article
Language
en
Open access
green

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CoChat. (2026). Citation check: Truly combining the advantages of polymeric and zeolite membranes for gas separations. https://app.cochat.ai/papers/10.1126/science.ade1411
The paper
Tan, X., Robijns, S., Thür, R., Ke, Q., De Witte, N., Lamaire, A., Li, Y., Aslam, I., Van Havere, D., Donckels, T., Van Assche, T., Van Speybroeck, V., Dusselier, M., & Vankelecom, I. (2022). Truly combining the advantages of polymeric and zeolite membranes for gas separations. Science. https://doi.org/10.1126/science.ade1411

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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).

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