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THE ANODIC OXIDATION OF AMMONIA AT PLATINUM BLACK ELECTRODES IN AQUEOUS KOH ELECTROLYTE
Abstract
Electrochemical kinetic studies are reported on the anodic oxidation of ammonia in aqueous potassium hydroxide solutions at platinum black electrodes. A kinetic scheme of consecutive reactions is proposed; Tafel slopes are deduced for various rate-determining mechanisms and compared with the experimental behavior. The reaction pathway is correlated with that involved in the analogous catalyzed ammonia vapor decomposition. The exchange currents obtained, compared with those for hydrogen oxidation, render the system unfavorable for fuel cell applications.
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Cited by
de Vooys, A. C. A., Koper, M. T. M., van Santen, R. A., & van Veen, J. A. R. (2001) · Journal of Electroanalytical Chemistry · doi:10.1016/s0022-0728(01)00491-0 · Cited by 441
Mechanism of electrochemical oxidation of ammonia
Bunce, N. J., & Bejan, D. (2011) · Electrochimica Acta · doi:10.1016/j.electacta.2011.07.078 · Cited by 255
Revisiting the electrochemical oxidation of ammonia on carbon-supported metal nanoparticle catalysts
Li, Z.-F., Wang, Y., & Botte, G. G. (2017) · Electrochimica Acta · doi:10.1016/j.electacta.2017.01.020 · Cited by 149
Green Chemistry: Advanced Electrocatalysts and System Design for Ammonia Oxidation
Tian, Y., Mao, Z., Wang, L., & Liang, J. (2023) · Small Structures · doi:10.1002/sstr.202200266 · Cited by 112
Recent Advances in Ammonia Electrolysis for Sustainable Hydrogen Generation
Babar, P., & Botte, G. G. (2024) · ACS Sustainable Chemistry & Engineering · doi:10.1021/acssuschemeng.4c02093 · Cited by 68
Metadata
- Authors
- Oswin, H. G., & Salomon, M.
- Venue
- Canadian Journal of Chemistry
- Publisher
- Canadian Science Publishing
- Published
- 1963-07-01
- Volume
- 41
- Issue
- 7
- Pages
- 1686-1694
- ISSN
- 0008-4042 (ISSN-L)
- 1480-3291
- OpenAlex
- W2018961683
- Cited by
- 238
- References
- 0
- FWCI
- 1.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- CoChat. (2026). Citation check: THE ANODIC OXIDATION OF AMMONIA AT PLATINUM BLACK ELECTRODES IN AQUEOUS KOH ELECTROLYTE. https://app.cochat.ai/papers/10.1139/v63-243
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- Oswin, H. G., & Salomon, M. (1963). THE ANODIC OXIDATION OF AMMONIA AT PLATINUM BLACK ELECTRODES IN AQUEOUS KOH ELECTROLYTE. Canadian Journal of Chemistry. https://doi.org/10.1139/v63-243
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