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New High Temperature Morphotropic Phase Boundary Piezoelectrics Based on Bi(Me)O3–PbTiO3 Ceramics
Abstract
New morphotropic phase boundary (MPB) piezoelectrics, with ferroelectric phase transition (T c) exceeding that of PbZrO 3–PbTiO 3 (PZT), were investigated. Based on a perovskite tolerance factor-T c relationship, new high T c MPB systems were projected in the Bi(Me)O 3–PbTiO 3 system, where Me is a relatively large B+3-site cation. For the (1-x)BiScO 3–(x)PbTiO 3 solid solution, a MPB was found at x-0.64 separating the rhombohedral and tetragonal phases, with correspondingly enhanced dielectric and piezoelectric properties. A transition temperature T c of ∼ 450°C was determined with evidence of T c's on the order of ≥ 600°C in the BiInO 3 and BiYbO 3 analogues, though issues of perovskite stability remain for the smaller tolerance end-member systems.
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Shannon, R. D. (1976) · Acta Crystallographica Section A · doi:10.1107/s0567739476001551 · Cited by 66,145
Cited by
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Gao, X., Yang, J., Wu, J., Xin, X., Li, Z., Yuan, X., Shen, X., & Dong, S. (2020) · Advanced Materials Technologies · doi:10.1002/admt.201900716 · Cited by 555
Fluorite-structure antiferroelectrics
Park, M. H., & Hwang, C. S. (2019) · Reports on Progress in Physics · doi:10.1088/1361-6633/ab49d6 · Cited by 69
Extrinsic contributions to piezoelectric Rayleigh behavior in morphotropic PbTiO3-BiScO3
Tutuncu, G., Forrester, J. S., Chen, J., & Jones, J. L. (2017) · Acta Materialia · doi:10.1016/j.actamat.2017.07.032 · Cited by 34
Metadata
- Authors
- Eitel, R. E., Randall, C. A., Shrout, T. R., Rehrig, P. W., Hackenberger, W., & Park, S.-E.
- Venue
- Japanese Journal of Applied Physics
- Publisher
- IOP Publishing
- Published
- 2001-10-01
- Volume
- 40
- Issue
- 10R
- Pages
- 5999
- ISSN
- 0021-4922 (ISSN-L)
- 1347-4065
- OpenAlex
- W2004245879
- Cited by
- 902
- References
- 1
- FWCI
- 13.48
- Type
- journal article
- Language
- en
- Open access
- closed
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- Eitel, R. E., Randall, C. A., Shrout, T. R., Rehrig, P. W., Hackenberger, W., & Park, S.-E. (2001). New High Temperature Morphotropic Phase Boundary Piezoelectrics Based on Bi(Me)O3–PbTiO3 Ceramics. Japanese Journal of Applied Physics. https://doi.org/10.1143/jjap.40.5999
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