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Rechargeable Lithium Sulfur Battery
Abstract
In this paper, the structural change of the sulfur cathode during the electrochemical reaction of a lithium sulfur battery employing 0.5 M LiCF 3 SO 3 -tetra(ethylene glycol) dimethyl ether (TEGDME) was studied by means of scanning electron microscopy (SEM), X-ray diffraction (XRD), and wave dispersive spectroscopy (WDS). The discharge process of the lithium sulfur cell could be divided in the first discharge region (2.4-2.1 V) where the reduction of elemental sulfur to form soluble polysulfides and further reduction of the soluble polysulfide occur, and the second discharge region (2.1-1.5 V) where the soluble polysulfides are reduced to form a nonuniform Li 2 S solid film covered over the carbon matrix. It was also found that the charge of lithium sulfur cell leads to the conversion from Li 2 S to the soluble polysulfide, resulting in the removal of Li 2 S layer formed on carbon matrix. However, the oxidization of the soluble polysulfide to solid sulfur hardly occurs and few Li 2 S are left on carbon matrix even at 100% depth of charge. © 2003 The Electrochemical Society. All rights reserved.
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Citations
Cited by
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Polysulfide Shuttle Study in the Li/S Battery System
Mikhaylik, Y. V., & Akridge, J. R. (2004) · Journal of The Electrochemical Society · doi:10.1149/1.1806394 · Cited by 2,115
Prospective materials and applications for Li secondary batteries
Jeong, G., Kim, Y.-U., Kim, H., Kim, Y.-J., & Sohn, H.-J. (2011) · Energy & Environmental Science · doi:10.1039/c0ee00831a · Cited by 616
Self-citationCarbon materials for Li–S batteries: Functional evolution and performance improvement
Liang, J., Sun, Z.-H., Li, F., & Cheng, H.-M. (2016) · Energy Storage Materials · doi:10.1016/j.ensm.2015.09.007 · Cited by 593
From lithium to sodium: Cell chemistry of room temperature sodium–air and sodium–sulfur batteries
Adelhelm, P., Hartmann, P., Bender, C. L., Busche, M., Eufinger, C., & Janek, J. (2015) · Beilstein Journal of Nanotechnology · doi:10.3762/bjnano.6.105 · Cited by 478
Metadata
- Authors
- Cheon, S.-E., Ko, K.-S., Cho, J.-H., Kim, S.-W., Chin, E.-Y., & Kim, H.-T.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2003
- Volume
- 150
- Issue
- 6
- Pages
- A796
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W1887039482
- Cited by
- 553
- References
- 0
- FWCI
- 5.03
- Type
- journal article
- Language
- en
- Open access
- closed
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- Cheon, S.-E., Ko, K.-S., Cho, J.-H., Kim, S.-W., Chin, E.-Y., & Kim, H.-T. (2003). Rechargeable Lithium Sulfur Battery. Journal of The Electrochemical Society. https://doi.org/10.1149/1.1571532
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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