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The Effect of Interfacial Deformation on Electrodeposition Kinetics
Abstract
Mullins-Sekerka linear stability analysis and the Barton and Bockris dendrite-propagation model are popular methods used to describe cathodic roughening and dendritic growth. These commonly cited theories employ kinetic relationships that differ in mathematical form, but both contain the effects of surface tension and local concentration deviations induced by surface roughening. Here, a kinetic model is developed which additionally includes mechanical forces such as elasticity, viscous drag, and pressure, showing their effect on exchange current densities and potentials at roughening interfaces. The proposed expression describes the current density in terms of applied overpotential at deformed interfaces with arbitrary three-dimensional interfacial geometry. Both the Mullins-Sekerka and the Barton-Bockris kinetics can be derived as special cases of the general expression, thereby validating the proposed model and elucidating the fundamental assumptions on which the two previous theories rely. © 2004 The Electrochemical Society. All rights reserved.
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Cites
Capacity Fade Mechanisms and Side Reactions in Lithium‐Ion Batteries
Arora, P., White, R. E., & Doyle, M. (1998) · Journal of The Electrochemical Society · doi:10.1149/1.1838857 · Cited by 1,408
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A review of lithium deposition in lithium-ion and lithium metal secondary batteries
Li, Z., Huang, J., Yann Liaw, B., Metzler, V., & Zhang, J. (2014) · Journal of Power Sources · doi:10.1016/j.jpowsour.2013.12.099 · Cited by 938
Koerver, R., Zhang, W., de Biasi, L., Schweidler, S., Kondrakov, A. O., Kolling, S., Brezesinski, T., Hartmann, P., Zeier, W. G., & Janek, J. (2018) · Energy & Environmental Science · doi:10.1039/c8ee00907d · Cited by 872
Stone, G. M., Mullin, S. A., Teran, A. A., Hallinan, D. T., Minor, A. M., Hexemer, A., & Balsara, N. P. (2012) · Journal of The Electrochemical Society · doi:10.1149/2.030203jes · Cited by 438
Mobile Ions in Composite Solids
Zou, Z., Li, Y., Lu, Z., Wang, D., Cui, Y., Guo, B., Li, Y., Liang, X., Feng, J., Li, H., et al. (2020) · Chemical Reviews · doi:10.1021/acs.chemrev.9b00760 · Cited by 348
Metadata
- Authors
- Monroe, C., & Newman, J.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2004
- Volume
- 151
- Issue
- 6
- Pages
- A880
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W2054983021
- Cited by
- 394
- References
- 1
- FWCI
- 1.96
- Type
- journal article
- Language
- en
- Open access
- closed
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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