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Effect of Agglomeration of Pt/C Catalyst on Hydrogen Peroxide Formation
Abstract
Various amounts of 20 wt % Pt/C catalysts ( 56.7 5.7 μ g carbon cm − 2 ) were loaded on glassy carbon (GC) disk electrode, and the effect of agglomeration on hydrogen peroxide formation in oxygen reduction was investigated by the rotating ring-disk electrode technique. The formation of H 2 O 2 was enhanced with a decrease in agglomeration of Pt/C. Even in the operating potential range of polymer electrolyte fuel cell cathodes (0.6-0.8 V), 10% hydrogen peroxide was formed at 5.7 μ g carbon cm − 2 Pt/C loaded on GC. These results revealed that series two-electron reduction pathway, which is negligible on clean bulk Pt surface, does exist on Pt particles supported on carbon. © 2004 The Electrochemical Society. All rights reserved.
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Markovic, N. M., Gasteiger, H. A., & Ross, P. N. (1995) · The Journal of Physical Chemistry · doi:10.1021/j100011a001 · Cited by 736
Cited by
High-Performance Electrocatalysts for Oxygen Reduction Derived from Polyaniline, Iron, and Cobalt
Wu, G., More, K. L., Johnston, C. M., & Zelenay, P. (2011) · Science · doi:10.1126/science.1200832 · Cited by 3,984
Understanding and approaches for the durability issues of Pt-based catalysts for PEM fuel cell
Shao, Y., Yin, G., & Gao, Y. (2007) · Journal of Power Sources · doi:10.1016/j.jpowsour.2007.07.004 · Cited by 1,197
Ren, P., Pei, P., Li, Y., Wu, Z., Chen, D., & Huang, S. (2020) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2020.100859 · Cited by 737
Zatoń, M., Rozière, J., & Jones, D. J. (2017) · Sustainable Energy & Fuels · doi:10.1039/c7se00038c · Cited by 435
Oezaslan, M., & Strasser, P. (2011) · Journal of Power Sources · doi:10.1016/j.jpowsour.2010.11.016 · Cited by 241
Metadata
- Authors
- Inaba, M., Yamada, H., Tokunaga, J., & Tasaka, A.
- Venue
- Electrochemical and Solid-State Letters
- Publisher
- The Electrochemical Society
- Published
- 2004
- Volume
- 7
- Issue
- 12
- Pages
- A474
- ISSN
- 1099-0062 (ISSN-L)
- OpenAlex
- W2135031573
- Cited by
- 224
- References
- 1
- FWCI
- 7.04
- Type
- journal article
- Language
- en
- Open access
- closed
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- Inaba, M., Yamada, H., Tokunaga, J., & Tasaka, A. (2004). Effect of Agglomeration of Pt/C Catalyst on Hydrogen Peroxide Formation. Electrochemical and Solid-State Letters. https://doi.org/10.1149/1.1814595
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