Cited by 1,205Advanced Battery Materials and TechnologiesAdvancements in Battery MaterialsBattery Modeling and Management

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Advanced Model for Solid Electrolyte Interphase Electrodes in Liquid and Polymer Electrolytes

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Peled, E., Golodnitsky, D., Ardel, G.·1997·Journal of The Electrochemical Society

DOI 10.1149/1.1837858

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Abstract

Recent studies show that the SEI on lithium and on anodes in liquid nonaqueous solutions consists of many different materials including , LiF, LiCl, , alkoxides, and nonconducting polymers. The equivalent circuit for such a mosaic‐type SEI electrode is extremely complex. It is shown that near room temperature the grain‐boundary resistance ( R gb ) for polyparticle solid electrolytes is larger than the bulk ionic resistance. Up to now, all models of SEI electrodes ignored the contribution of R gb to the overall SEI resistance. We show here that this neglect has no justification. On the basis of recent results, we propose here for SEI electrodes equivalent circuits which take into account the contribution of grain‐boundary and other interfacial impedance terms. This model accounts for a variety of different types of Nyquist plots reported for lithium and electrodes in liquid nonaqueous and polymer electrolytes.

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Research works printed but not linked: 14

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“Thick fibrous mats will result in the formation of a thick SEI layer at the first cycle thus, resulting in high capacity loss at the first cycle and low capacity retention [57].”
BackgroundInfluential
Organosulfur Compounds Enable Uniform Lithium Plating and Long-Term Battery Cycling Stability
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“As for the spatial distribution of SEI, a mosaic-like SEI model is widely accepted [33, 49], in which inorganic components may be closer to metal potassium anode surfaces [28, 50].”
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“Nowadays, it is generally accepted that the mainstream structures of the SEI are the double layer model 23,24 and the mosaic model, 25 both validated by cryogenic electron microscopy (cryo-EM).”
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Direct Evidence of LiF Formation at Electrode/Electrolyte Interface by 7Li and 19F Double-Resonance Solid-State NMR Spectroscopy
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Structure and evolution of solid electrolyte interphase (SEI) at the electrode-electrolyte interface
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Review of Local In Situ Probing Techniques for the Interfaces of Lithium‐Ion and Lithium–Oxygen Batteries
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Authors: Peled, E., Golodnitsky, D., & Ardel, G.
Affiliations: Tel Aviv University (IL)
ORCID: Peled, E.
Golodnitsky, D.
Venue: Journal of The Electrochemical Society
Publisher: The Electrochemical Society
Published: 1997-08-01
Volume: 144
Issue: 8
Pages: L208-L210
ISSN: 0013-4651 (ISSN-L)
1945-7111
DOI: 10.1149/1.1837858
OpenAlex: W2037447290
Cited by: 1,205
References: 0
Citations by year: 2026: 86 · 2025: 96 · 2024: 110 · 2023: 119 · 2022: 99 · 2021: 129 · 2020: 107 · 2019: 88 · 2018: 65 · 2017: 51 · 2016: 32 · 2015: 37 · 2014: 37 · 2013: 21 · 2012: 25
FWCI: 4.51
Type: journal article
Language: en
Open access: bronze
doi.org
Licence: iopscience.iop.org/page/copyright (vor, 8162 d)
iopscience.iop.org/info/page/text-and-data-mining (tdm, 8162 d)
Locations: Journal of The Electrochemical Society (publishedVersion)
Funders: Tel Aviv University
Ministry of Defense
U.S. Air Force
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
Physical Sciences › Engineering › Automotive Engineering › Battery Modeling and Management
Keywords: solid electrolyte interphase, grain boundary resistance, interfacial impedance, lithium metal anode, lithium-ion batteries, polymer electrolytes, Nyquist plot, lithium fluoride

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Advanced Model for Solid Electrolyte Interphase Electrodes in Liquid and Polymer Electrolytes

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