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Lithium‐Ion Cells with Aqueous Electrolytes
Abstract
The electrochemical intercalation of lithium can occur in aqueous electrolytes provided that the host material, the Li + ion concentration and the pH, are carefully selected. Therefore, rechargeable cells with aqueous electrolytes based on the intercalation of lithium in both electrodes can be made. Here we describe some examples of these cells including Li 1 − x Mn 2 O 4 / Li 1 + x Mn 2 O 4 , Li 1 − x Mn 2 O 4 / γ ‐ Li 0.36 MnO 2 , and LiMn 2 O 4 / VO 2 ( B ) using several aqueous electrolytes. The voltage vs. charge relation for these aqueous cells predicted from the difference of the voltages of Li / LiMn 2 O 4 , Li / γ ‐ Li 0.36 MnO 2 , and Li / VO 2 ( B ) nonaqueous cells is in excellent agreement with experiment, proving that lithium intercalation is occurring in the cells with aqueous electrolytes. The cells have poor cycle life (approximately 25 cycles) for reasons that are not yet understood.
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Cited by
Layered vanadium and molybdenum oxides: batteries and electrochromics
Chernova, N. A., Roppolo, M., Dillon, A. C., & Whittingham, M. S. (2009) · Journal of Materials Chemistry · doi:10.1039/b819629j · Cited by 874
Recent Progress in Aqueous Lithium‐Ion Batteries
Wang, Y., Yi, J., & Xia, Y. (2012) · Advanced Energy Materials · doi:10.1002/aenm.201200065 · Cited by 594
Ramanujapuram, A., & Yushin, G. (2018) · Advanced Energy Materials · doi:10.1002/aenm.201802624 · Cited by 130
Metadata
- Authors
- Li, W., & Dahn, J. R.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1995-06-01
- Volume
- 142
- Issue
- 6
- Pages
- 1742-1746
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2057811098
- Cited by
- 198
- References
- 0
- FWCI
- 4.31
- Type
- journal article
- Language
- en
- Open access
- closed
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- Li, W., & Dahn, J. R. (1995). Lithium‐Ion Cells with Aqueous Electrolytes. Journal of The Electrochemical Society. https://doi.org/10.1149/1.2044187
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