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Electrochemistry of Pyrite‐Based Cathodes for Ambient Temperature Lithium Batteries
Open accessAbstract
The charge and discharge mechanisms of and cells near room temperature are studied by in situ x‐ray diffraction and in situ 57 Fe Mössbauer spectroscopy. The electrochemical behavior of these cells are compared, and their cell reactions are described. For , the cycling behavior of is reversible. However, for , structural decomposition of occurs, and disproportionation to nonstoichiometric and S is observed. Similarly, when cells are recharged to 2.8V, the cathode is a mixture of and S. Examination of the mixture by differential scanning calorimetry shows that and S react to form above 200°C. This explains why high temperature cells cycle reversibly while ambient temperature cells show poor reversibility.
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Cited by
Cabana, J., Monconduit, L., Larcher, D., & Palacín, M. R. (2010) · Advanced Materials · doi:10.1002/adma.201000717 · Cited by 2,361
Luo, K., Roberts, M. R., Hao, R., Guerrini, N., Pickup, D. M., Liu, Y.-S., Edström, K., Guo, J., Chadwick, A. V., Duda, L. C., et al. (2016) · Nature Chemistry · doi:10.1038/nchem.2471 · Cited by 1,241
Electrode Degradation in Lithium-Ion Batteries
Pender, J. P., Jha, G., Youn, D. H., Ziegler, J. M., Andoni, I., Choi, E. J., Heller, A., Dunn, B. S., Weiss, P. S., Penner, R. M., et al. (2020) · ACS Nano · doi:10.1021/acsnano.9b04365 · Cited by 873
Pyrite FeS2for high-rate and long-life rechargeable sodium batteries
Hu, Z., Zhu, Z., Cheng, F., Zhang, K., Wang, J., Chen, C., & Chen, J. (2015) · Energy & Environmental Science · doi:10.1039/c4ee03759f · Cited by 686
Design strategies for nonaqueous multivalent-ion and monovalent-ion battery anodes
Li, M., Lu, J., Ji, X., Li, Y., Shao, Y., Chen, Z., Zhong, C., & Amine, K. (2020) · Nature Reviews Materials · doi:10.1038/s41578-019-0166-4 · Cited by 438
Metadata
- Authors
- Fong, R., Dahn, J. R., & Jones, C. H. W.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1989-11-01
- Volume
- 136
- Issue
- 11
- Pages
- 3206-3210
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2105745725
- Cited by
- 167
- References
- 0
- FWCI
- 0.94
- Type
- journal article
- Language
- en
- Open access
- bronze
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- CoChat. (2026). Citation check: Electrochemistry of Pyrite‐Based Cathodes for Ambient Temperature Lithium Batteries. https://app.cochat.ai/papers/10.1149/1.2096426
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- Fong, R., Dahn, J. R., & Jones, C. H. W. (1989). Electrochemistry of Pyrite‐Based Cathodes for Ambient Temperature Lithium Batteries. Journal of The Electrochemical Society. https://doi.org/10.1149/1.2096426
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