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Carbon Dioxide Reduction at a Metal Phthalocyanine Catalyzed Carbon Electrode
Open accessAbstract
Metal phthalocyanines deposited on carbon electrodes have been found to catalyze the electroreduction of carbon dioxide to formic acid in acid solutions . The overpotential for reduction on cobalt phthalocyanine is approximately 200 mV lower than on the best metal cathodes at currents up to 10 mA/cm 2 . The main reaction product in long‐term electrolysis is the formate ion at . Methanol is also produced at lower p H values. The phthalocyanine becomes inactive in the less acid solutions once a fairly negative potential is imposed, probably due to an irreversible reduction of the catalyst.
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Cited by
A review of catalysts for the electroreduction of carbon dioxide to produce low-carbon fuels
Qiao, J., Liu, Y., Hong, F., & Zhang, J. (2014) · Chem. Soc. Rev. · doi:10.1039/c3cs60323g · Cited by 2,990
Domino electroreduction of CO2 to methanol on a molecular catalyst
Wu, Y., Jiang, Z., Lu, X., Liang, Y., & Wang, H. (2019) · Nature · doi:10.1038/s41586-019-1760-8 · Cited by 1,194
Electro- and Solar-Driven Fuel Synthesis with First Row Transition Metal Complexes
Dalle, K. E., Warnan, J., Leung, J. J., Reuillard, B., Karmel, I. S., & Reisner, E. (2019) · Chemical Reviews · doi:10.1021/acs.chemrev.8b00392 · Cited by 912
Hawecker, J., Lehn, J., & Ziessel, R. (1986) · Helvetica Chimica Acta · doi:10.1002/hlca.19860690824 · Cited by 688
Electrocatalytic reduction of carbon dioxide: opportunities with heterogeneous molecular catalysts
Sun, L., Reddu, V., Fisher, A. C., & Wang, X. (2020) · Energy & Environmental Science · doi:10.1039/c9ee03660a · Cited by 452
Metadata
- Authors
- Kapusta, S., & Hackerman, N.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1984-07-01
- Volume
- 131
- Issue
- 7
- Pages
- 1511-1514
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2013116501
- Cited by
- 168
- References
- 0
- FWCI
- 6.96
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Kapusta, S., & Hackerman, N. (1984). Carbon Dioxide Reduction at a Metal Phthalocyanine Catalyzed Carbon Electrode. Journal of The Electrochemical Society. https://doi.org/10.1149/1.2115882
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
Semantic Scholar’s data is described in: Kinney, R., et al. (2023). The Semantic Scholar Open Data Platform. arXiv:2301.10140.
