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A Lithium/Dissolved Sulfur Battery with an Organic Electrolyte
Abstract
Prototype cells of the configuration Li/∼5M S as Li 2 S n , THF, 1 M LiAsF 6 / C have been characterized with regard to capacity, rate, and rechargeability. Virtually 100% of the theoretical capacity could be realized at 50°C at rates below 1.0 mA/cm 2 . In high rate cell configurations, 75% cathode utilization is possible at ∼4 mA/cm 2 (C/3–C/4 rate). The capacities at high rate are enhanced by Lewis acids, although the ultimate cause of rate limitation is passivation of the current collector by discharge products. The self‐discharge rates of Li in contact with 4–5M S (as Li 2 S n ) solutions reveal capacity losses of 0.5%/day at 25°C to 4.4%/day at 71°C. Based on the experimental results, a practical energy density of ∼300 W‐hr kg −1 is possible using a standard cell design. Results on the battery's rechargeability are briefly reviewed.
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Cited by
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Lithium Batteries: Status, Prospects and Future
Scrosati, B., & Garche, J. (2010) · Journal of Power Sources · doi:10.1016/j.jpowsour.2009.11.048 · Cited by 5,153
Challenges and Prospects of Lithium–Sulfur Batteries
Manthiram, A., Fu, Y., & Su, Y.-S. (2013) · Accounts of Chemical Research · doi:10.1021/ar300179v · Cited by 2,380
Polysulfide Shuttle Study in the Li/S Battery System
Mikhaylik, Y. V., & Akridge, J. R. (2004) · Journal of The Electrochemical Society · doi:10.1149/1.1806394 · Cited by 2,115
Placke, T., Kloepsch, R., Dühnen, S., & Winter, M. (2017) · Journal of Solid State Electrochemistry · doi:10.1007/s10008-017-3610-7 · Cited by 1,117
Metadata
- Authors
- Rauh, R. D., Abraham, K. M., Pearson, G. F., Surprenant, J. K., & Brummer, S. B.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 1979-04-01
- Volume
- 126
- Issue
- 4
- Pages
- 523-527
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2124235175
- Cited by
- 592
- References
- 0
- FWCI
- 2.93
- Type
- journal article
- Language
- en
- Open access
- closed
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- Rauh, R. D., Abraham, K. M., Pearson, G. F., Surprenant, J. K., & Brummer, S. B. (1979). A Lithium/Dissolved Sulfur Battery with an Organic Electrolyte. Journal of The Electrochemical Society. https://doi.org/10.1149/1.2129079
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