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On the Surface Chemical Aspects of Very High Energy Density, Rechargeable Li–Sulfur Batteries
Open accessAbstract
Li(metal)–sulfur (Li–S) systems are among the rechargeable batteries of the highest possible energy density due to the high capacity of both electrodes. The surface chemistry developed on Li electrodes in electrolyte solutions for Li–S batteries was rigorously studied using Fourier transform infrared and X-ray photoelectron spectroscopies. A special methodology was developed for handling the highly reactive Li samples. It was possible to analyze the contribution of solvents such as 1-3 dioxolane, the electrolyte , polysulfide , and additives to protective surface films that are formed on the Li electrodes. The role of as a critical component whose presence in solutions prevents a shuttle mechanism that limits the capacity of the sulfur electrodes is discussed and explained herein.
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Citations
Cites
Spectrometric Identification of Organic Compounds
Silverstein, R. M., & Bassler, G. C. (1962) · Journal of Chemical Education · doi:10.1021/ed039p546 · Cited by 14,272
Cited by
Li-O2 and Li-S batteries with high energy storage
Bruce, P. G., Freunberger, S. A., Hardwick, L. J., & Tarascon, J.-M. (2012) · Nature Materials · doi:10.1038/nmat3191 · Cited by 9,479
Reviving the lithium metal anode for high-energy batteries
Lin, D., Liu, Y., & Cui, Y. (2017) · Nature Nanotechnology · doi:10.1038/nnano.2017.16 · Cited by 6,763
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Challenges and Prospects of Lithium–Sulfur Batteries
Manthiram, A., Fu, Y., & Su, Y.-S. (2013) · Accounts of Chemical Research · doi:10.1021/ar300179v · Cited by 2,380
Wang, H., Yang, Y., Liang, Y., Robinson, J. T., Li, Y., Jackson, A., Cui, Y., & Dai, H. (2011) · Nano Letters · doi:10.1021/nl200658a · Cited by 2,119
Metadata
- Authors
- Aurbach, D., Pollak, E., Elazari, R., Salitra, G., Kelley, C. S., & Affinito, J.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2009
- Volume
- 156
- Issue
- 8
- Pages
- A694
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W2057899803
- Cited by
- 1,443
- References
- 1
- FWCI
- 20.06
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Aurbach, D., Pollak, E., Elazari, R., Salitra, G., Kelley, C. S., & Affinito, J. (2009). On the Surface Chemical Aspects of Very High Energy Density, Rechargeable Li–Sulfur Batteries. Journal of The Electrochemical Society. https://doi.org/10.1149/1.3148721
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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