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A Dusty Fluid Model for Predicting Hydroxyl Anion Conductivity in Alkaline Anion Exchange Membranes
Open accessAbstract
Advances in metal-cation-free, quaternary ammonium, polymer alkaline anion exchange membranes ͑AAEMs͒ have provided a recent resurgence of interest in the alkaline fuel cell ͑AFC͒.The alkaline environment supported by the AAEM offers several potential advantages, including opportunities for the use of non-noble metal catalysts with high energy density and logistically favorable fuels and oxidants, such as methanol and air.However, recent experimental literature has shown that the AAEM derived AFCs have considerable resistive losses that can be attributed to the AAEM.This work describes a dusty fluid model used to predict AAEM conductivities as a function of relative humidity and membrane properties in an initial attempt at forming a framework for understanding the processes at work.A percolation model is used to account for the membrane structure.The model is validated using Nafion 115 conductivity data.
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Cites
Proton Transfer 200 Years after von Grotthuss: Insights from Ab Initio Simulations
Marx, D. (2006) · ChemPhysChem · doi:10.1002/cphc.200600128 · Cited by 920
Transport in Polymer-Electrolyte Membranes
Weber, A. Z., & Newman, J. (2004) · Journal of The Electrochemical Society · doi:10.1149/1.1639157 · Cited by 462
Transport in Polymer-Electrolyte Membranes
Weber, A. Z., & Newman, J. (2003) · Journal of The Electrochemical Society · doi:10.1149/1.1580822 · Cited by 411
Cited by
Anion-exchange membranes in electrochemical energy systems
Varcoe, J. R., Atanassov, P., Dekel, D. R., Herring, A. M., Hickner, M. A., Kohl, P. A., Kucernak, A. R., Mustain, W. E., Nijmeijer, K., Scott, K., et al. (2014) · Energy Environ. Sci. · doi:10.1039/c4ee01303d · Cited by 2,051
Selectivity of ion exchange membranes: A review
Luo, T., Abdu, S., & Wessling, M. (2018) · Journal of Membrane Science · doi:10.1016/j.memsci.2018.03.051 · Cited by 1,123
Towards membrane-electrode assembly systems for CO2 reduction: a modeling study
Weng, L.-C., Bell, A. T., & Weber, A. Z. (2019) · Energy & Environmental Science · doi:10.1039/c9ee00909d · Cited by 452
Metadata
- Authors
- Grew, K. N., & Chiu, W. K. S.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2010
- Volume
- 157
- Issue
- 3
- Pages
- B327
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W2102365354
- Cited by
- 212
- References
- 3
- FWCI
- 3.99
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Grew, K. N., & Chiu, W. K. S. (2010). A Dusty Fluid Model for Predicting Hydroxyl Anion Conductivity in Alkaline Anion Exchange Membranes. Journal of The Electrochemical Society. https://doi.org/10.1149/1.3273200
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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