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In Situ Measurements of Stress-Potential Coupling in Lithiated Silicon
Open accessAbstract
An analysis of the dependence of electric potential on the state of stress of a lithiated-silicon electrode is presented. Based on the Larché and Cahn chemical potential for a solid solution, a thermodynamic argument is made for the existence of the stress-potential coupling in lithiated silicon; based on the known properties of the material, the magnitude of the coupling is estimated to be ∼ 60 mV / GPa in thin-film geometry. An experimental investigation is carried out on silicon thin-film electrodes in which the stress is measured in situ during electrochemical lithiation and delithiation. By progressively varying the stress through incremental delithiation, the relation between stress change and electric-potential change is measured to be 100–120 mV/GPa, which is of the same order of magnitude as the prediction of the analysis. The importance of the coupling is discussed in interpreting the hysteresis observed in the potential vs state-of-charge plots and the role of stress in modifying the maximum charge capacity of a silicon electrode under stress.
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Cites
Stress generation and fracture in lithium insertion materials
Christensen, J., & Newman, J. (2006) · Journal of Solid State Electrochemistry · doi:10.1007/s10008-006-0095-1 · Cited by 727
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Nie, M., Abraham, D. P., Chen, Y., Bose, A., & Lucht, B. L. (2013) · The Journal of Physical Chemistry C · doi:10.1021/jp404155y · Cited by 578
A comparison of methodologies for the non-invasive characterisation of commercial Li-ion cells
Barai, A., Uddin, K., Dubarry, M., Somerville, L., McGordon, A., Jennings, P., & Bloom, I. (2019) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2019.01.001 · Cited by 319
Tahmasebi, M. H., Kramer, D., Geßwein, H., Zheng, T., Leung, K.-C., Lo, B. T. W., Mönig, R., & Boles, S. T. (2020) · Journal of Materials Chemistry A · doi:10.1039/c9ta13745a · Cited by 31
Metadata
- Authors
- Sethuraman, V. A., Srinivasan, V., Bower, A. F., & Guduru, P. R.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2010
- Volume
- 157
- Issue
- 11
- Pages
- A1253
- ISSN
- 0013-4651 (ISSN-L)
- OpenAlex
- W2170656604
- Cited by
- 364
- References
- 1
- FWCI
- 9.22
- Type
- journal article
- Language
- en
- Open access
- green
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- Sethuraman, V. A., Srinivasan, V., Bower, A. F., & Guduru, P. R. (2010). In Situ Measurements of Stress-Potential Coupling in Lithiated Silicon. Journal of The Electrochemical Society. https://doi.org/10.1149/1.3489378
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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