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Investigation of the Solid Electrolyte Interphase Formed by Fluoroethylene Carbonate on Si Electrodes
Open accessAbstract
The solid electrolyte interphase (SEI) formed by a fluoroethylene carbonate (FEC)-based electrolyte on a Si electrode was investigated using X-ray photoelectron spectroscopy (XPS) and time of flight–secondary ion mass spectrometry (ToF-SIMS). The FEC-derived SEI consists of lithium fluoride and a polyene-compound, which are originated from free fluoride and the acetylene unit due to the preferential reaction of FEC, and is very thin. Oxidation of the Si electrode of the EC-based cell was confirmed, although it did not proceed to a significant extent. The FEC-derived SEI protects against not only the decomposition of the FEC-based electrolyte, but also oxidation of the Si electrode. The FEC-derived SEI acts as a passivation film for the Si electrode, which results in the improvement of the cycling performance.
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Citations
Cited by
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Challenges Facing Lithium Batteries and Electrical Double‐Layer Capacitors
Choi, N., Chen, Z., Freunberger, S. A., Ji, X., Sun, Y., Amine, K., Yushin, G., Nazar, L. F., Cho, J., & Bruce, P. G. (2012) · Angewandte Chemie International Edition · doi:10.1002/anie.201201429 · Cited by 2,700
Negative electrodes for Na-ion batteries
Dahbi, M., Yabuuchi, N., Kubota, K., Tokiwa, K., & Komaba, S. (2014) · Physical Chemistry Chemical Physics · doi:10.1039/c4cp00826j · Cited by 623
Artificial Protection Film on Lithium Metal Anode toward Long‐Cycle‐Life Lithium–Oxygen Batteries
Liu, Q., Xu, J., Yuan, S., Chang, Z., Xu, D., Yin, Y., Li, L., Zhong, H., Jiang, Y., Yan, J., et al. (2015) · Advanced Materials · doi:10.1002/adma.201501490 · Cited by 482
Waldmann, T., Iturrondobeitia, A., Kasper, M., Ghanbari, N., Aguesse, F., Bekaert, E., Daniel, L., Genies, S., Gordon, I. J., Löble, M. W., et al. (2016) · Journal of The Electrochemical Society · doi:10.1149/2.1211609jes · Cited by 328
Metadata
- Authors
- Nakai, H., Kubota, T., Kita, A., & Kawashima, A.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2011-05-05
- Volume
- 158
- Issue
- 7
- Pages
- A798-A801
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2142015025
- Cited by
- 360
- References
- 0
- FWCI
- 17.83
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Nakai, H., Kubota, T., Kita, A., & Kawashima, A. (2011). Investigation of the Solid Electrolyte Interphase Formed by Fluoroethylene Carbonate on Si Electrodes. Journal of The Electrochemical Society. https://doi.org/10.1149/1.3589300
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