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Survey of Gas Expansion in Li-Ion NMC Pouch Cells
Open accessAbstract
This preliminary study investigates initial gas formation in Li[Ni 0.4 Mn 0.4 Co 0.2 ]O 2 (NMC442) pouch cells with three different electrolytes: 3:7 ethylene carbonate : ethyl methyl carbonate (EC:EMC) w/ 1 M LiPF 6 as the control, control + 2% prop-1-ene-1,3-sultone (PES) and control + 2% vinylene carbonate (VC). In situ volume measurements reveal three main features of gas evolution, an initial gas step, gas absorption, and a second gas step at higher voltage. Gas chromatography-mass spectrometry is employed to identify the gaseous compounds. This work illustrates the strong dependence of volume change due to gas evolution on additives, charging rate and temperature.
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Cited by
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Mrozik, W., Rajaeifar, M. A., Heidrich, O., & Christensen, P. (2021) · Energy & Environmental Science · doi:10.1039/d1ee00691f · Cited by 1,028
Li plating as unwanted side reaction in commercial Li-ion cells – A review
Waldmann, T., Hogg, B.-I., & Wohlfahrt-Mehrens, M. (2018) · Journal of Power Sources · doi:10.1016/j.jpowsour.2018.02.063 · Cited by 895
Electrolyte Oxidation Pathways in Lithium-Ion Batteries
Rinkel, B. L. D., Hall, D. S., Temprano, I., & Grey, C. P. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c06363 · Cited by 455
Waldmann, T., Iturrondobeitia, A., Kasper, M., Ghanbari, N., Aguesse, F., Bekaert, E., Daniel, L., Genies, S., Gordon, I. J., Löble, M. W., et al. (2016) · Journal of The Electrochemical Society · doi:10.1149/2.1211609jes · Cited by 328
Roadmap for a sustainable circular economy in lithium-ion and future battery technologies
Harper, G. D. J., Kendrick, E., Anderson, P. A., Mrozik, W., Christensen, P., Lambert, S., Greenwood, D., Das, P. K., Ahmeid, M., Milojevic, Z., et al. (2023) · Journal of Physics: Energy · doi:10.1088/2515-7655/acaa57 · Cited by 137
Metadata
- Authors
- Self, J., Aiken, C. P., Petibon, R., & Dahn, J. R.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2015
- Volume
- 162
- Issue
- 6
- Pages
- A796-A802
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2161465156
- Cited by
- 166
- References
- 0
- FWCI
- 21.85
- Type
- journal article
- Language
- en
- Open access
- hybrid
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- Self, J., Aiken, C. P., Petibon, R., & Dahn, J. R. (2015). Survey of Gas Expansion in Li-Ion NMC Pouch Cells. Journal of The Electrochemical Society. https://doi.org/10.1149/2.0081506jes
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