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Studies of Li-Air Cells Utilizing Dimethyl Sulfoxide-Based Electrolyte
Open accessAbstract
Dimethyl Sulfoxide (DMSO) was evaluated as a practical solvent for the rechargeable lithium air battery. Redox characteristics of the dissolved oxygen and its reduction products in the presence of lithium hexafluorophosphate (LiPF 6 ) supporting electrolyte were studied via cyclic, rotating disk (RDE) and ring-disk (RRDE) electrode voltammetry. The DMSO medium facilitates reversible reduction and oxidation processes in contrast to other solvent-based electrolytes studied. Galvanostatic discharge-charge cycling of the Li-O 2 cells has shown characteristics of rechargeability expected from voltammetric studies. Multiple high-efficiency discharge-charge cycles are possible if the depth of discharge of the carbon cathode is limited to avoid excessive passivation by the discharge products. The discharge voltage of this Li-O 2 cell is higher than cells assembled with other non-aqueous organic electrolytes, an attribute ascribed to the stability of superoxide (O 2 − ), the one-electron reduction product of oxygen.
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Citations
Cited by
Electrolytes and Interphases in Li-Ion Batteries and Beyond
Xu, K. (2014) · Chemical Reviews · doi:10.1021/cr500003w · Cited by 5,566
Charging a Li–O2 battery using a redox mediator
Chen, Y., Freunberger, S. A., Peng, Z., Fontaine, O., & Bruce, P. G. (2013) · Nature Chemistry · doi:10.1038/nchem.1646 · Cited by 937
A review of cathode materials and structures for rechargeable lithium–air batteries
Ma, Z., Yuan, X., Li, L., Ma, Z.-F., Wilkinson, D. P., Zhang, L., & Zhang, J. (2015) · Energy & Environmental Science · doi:10.1039/c5ee00838g · Cited by 485
From lithium to sodium: Cell chemistry of room temperature sodium–air and sodium–sulfur batteries
Adelhelm, P., Hartmann, P., Bender, C. L., Busche, M., Eufinger, C., & Janek, J. (2015) · Beilstein Journal of Nanotechnology · doi:10.3762/bjnano.6.105 · Cited by 478
A Solution-Phase Bifunctional Catalyst for Lithium–Oxygen Batteries
Sun, D., Shen, Y., Zhang, W., Yu, L., Yi, Z., Yin, W., Wang, D., Huang, Y., Wang, J., Wang, D., et al. (2014) · Journal of the American Chemical Society · doi:10.1021/ja501877e · Cited by 466
Metadata
- Authors
- Trahan, M. J., Mukerjee, S., Plichta, E. J., Hendrickson, M. A., & Abraham, K. M.
- Venue
- Journal of The Electrochemical Society
- Publisher
- The Electrochemical Society
- Published
- 2012-12-04
- Volume
- 160
- Issue
- 2
- Pages
- A259-A267
- ISSN
- 0013-4651 (ISSN-L)
- 1945-7111
- OpenAlex
- W2043738058
- Cited by
- 272
- References
- 0
- FWCI
- 20.75
- Type
- journal article
- Language
- en
- Open access
- bronze
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- Trahan, M. J., Mukerjee, S., Plichta, E. J., Hendrickson, M. A., & Abraham, K. M. (2013). Studies of Li-Air Cells Utilizing Dimethyl Sulfoxide-Based Electrolyte. Journal of The Electrochemical Society. https://doi.org/10.1149/2.048302jes
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Contains information from the Semantic Scholar Academic Graph Datasets, made available under the ODC Attribution License (ODC-BY 1.0).
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