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Comparative Study on Adhesive Performance of Functional Monomers
Abstract
Mild self-etch adhesives demineralize dentin only partially, leaving hydroxyapatite around collagen within a submicron hybrid layer. We hypothesized that this residual hydroxyapatite may serve as a receptor for chemical interaction with the functional monomer and, subsequently, contribute to adhesive performance in addition to micro-mechanical hybridization. We therefore chemically characterized the adhesive interaction of 3 functional monomers with synthetic hydroxyapatite, using x-ray photoelectron spectroscopy and atomic absorption spectrophotometry. We further characterized their interaction with dentin ultra-morphologically, using transmission electron microscopy. The monomer 10-methacryloxydecyl dihydrogen phosphate (10-MDP) readily adhered to hydroxyapatite. This bond appeared very stable, as confirmed by the low dissolution rate of its calcium salt in water. The bonding potential of 4-methacryloxyethyl trimellitic acid (4-MET) was substantially lower. The monomer 2-methacryloxyethyl phenyl hydrogen phosphate (phenyl-P) and its bond to hydroxyapatite did not appear to be hydrolytically stable. Besides self-etching dentin, specific functional monomers have additional chemical bonding efficacy that is expected to contribute to their adhesive potential to tooth tissue.
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Citations
Cited by
Peumans, M., De Munck, J., Van Landuyt, K. L., Poitevin, A., Lambrechts, P., & Van Meerbeek, B. (2010) · Dental Materials · doi:10.1016/j.dental.2010.08.190 · Cited by 301
Self-citationPeumans, M., De Munck, J., Mine, A., & Van Meerbeek, B. (2014) · Dental Materials · doi:10.1016/j.dental.2014.07.007 · Cited by 299
Self-citationDevelopment of an antibacterial root canal filling system containing MDPB
Kitagawa, R., Kitagawa, H., Izutani, N., Hirose, N., Hayashi, M., & Imazato, S. (2014) · Journal of Dental Research · doi:10.1177/0022034514549808 · Cited by 31
Dentine disorders and adhesive treatments: A systematic review
Massé, L., Etienne, O., Noirrit-Esclassan, E., Bailleul-Forestier, I., & Garot, E. (2021) · Journal of Dentistry · doi:10.1016/j.jdent.2021.103654 · Cited by 25
Metadata
- Authors
- Yoshida, Y., Nagakane, K., Fukuda, R., Nakayama, Y., Okazaki, M., Shintani, H., Inoue, S., Tagawa, Y., Suzuki, K., De Munck, J., & Van Meerbeek, B.
- Venue
- Journal of Dental Research
- Publisher
- SAGE Publications
- Published
- 2004-06
- Volume
- 83
- Issue
- 6
- Pages
- 454-458
- ISSN
- 0022-0345 (ISSN-L)
- 1544-0591
- OpenAlex
- W2148451900
- Cited by
- 1,188
- References
- 0
- FWCI
- 47.04
- Type
- journal article
- Language
- en
- Open access
- closed
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- Yoshida, Y., Nagakane, K., Fukuda, R., Nakayama, Y., Okazaki, M., Shintani, H., Inoue, S., Tagawa, Y., Suzuki, K., De Munck, J., & Van Meerbeek, B. (2004). Comparative Study on Adhesive Performance of Functional Monomers. Journal of Dental Research. https://doi.org/10.1177/154405910408300604
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