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Photoinduced Oxyamination of Enamines and Aldehydes with TEMPO Catalyzed by [Ru(bpy)3]2+
Abstract
Tris(bipyridyl)ruthenium(II) ([Ru(bpy)3]2+: TB(II)) catalyzes oxidative coupling of enamines and aldehydes with 2,2,6,6-tetramethylpiperidinyl-1-oxy (TEMPO) under irradiation of visible light to afford α-oxyaminated carbonyl compounds. The visible light irradiation is essential to generate the triplet excited state of ∗TB(II) which acts as an oxidizing agent. This is a new procedure for radical coupling based on single electron transfer mediated by photoactivated TB.
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Citations
Cited by
Prier, C. K., Rankic, D. A., & MacMillan, D. W. C. (2013) · Chemical Reviews · doi:10.1021/cr300503r · Cited by 9,590
Dual Catalysis Strategies in Photochemical Synthesis
Skubi, K. L., Blum, T. R., & Yoon, T. P. (2016) · Chemical Reviews · doi:10.1021/acs.chemrev.6b00018 · Cited by 2,686
Visible light photocatalysis as a greener approach to photochemical synthesis
Yoon, T. P., Ischay, M. A., & Du, J. (2010) · Nature Chemistry · doi:10.1038/nchem.687 · Cited by 2,657
Photoredox Catalysis with Visible Light
Zeitler, K. (2009) · Angewandte Chemie International Edition · doi:10.1002/anie.200904056 · Cited by 991
Photoredox-Catalyzed C–H Functionalization Reactions
Holmberg-Douglas, N., & Nicewicz, D. A. (2022) · Chemical Reviews · doi:10.1021/acs.chemrev.1c00311 · Cited by 989
Metadata
- Authors
- Koike, T., & Akita, M.
- Venue
- Chemistry Letters
- Publisher
- Oxford University Press (OUP)
- Published
- 2009-01-17
- Volume
- 38
- Issue
- 2
- Pages
- 166-167
- ISSN
- 0366-7022 (ISSN-L)
- 1348-0715
- OpenAlex
- W2951782980
- Cited by
- 165
- References
- 0
- FWCI
- 11.33
- Type
- journal article
- Language
- en
- Open access
- closed
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- Koike, T., & Akita, M. (2009). Photoinduced Oxyamination of Enamines and Aldehydes with TEMPO Catalyzed by [Ru(bpy)3]2+. Chemistry Letters. https://doi.org/10.1246/cl.2009.166
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