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Time-domain mid-infrared frequency-comb spectrometer
Abstract
A novel type of Fourier-transform infrared spectrometer (FTIR) is demonstrated. It is based on two Ti:sapphire lasers emitting femtosecond pulse trains with slightly different repetition frequencies. Two mid-infrared beams-derived from those lasers by rectification in GaSe-are superimposed upon a detector to produce purely time-domain interferograms that encode the infrared spectrum. The advantages of this spectrometer compared with the common FTIR include ease of operation (no moving parts), speed of acquisition (100 micros demonstrated), and not-yet-shown collimated long-distance propagation, diffraction-limited microscopic probing, and electronically controllable chemometric factoring. Extending time-domain frequency-comb spectroscopy to lower (terahertz) or higher (visible, ultraviolet) frequencies should be feasible.
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Metadata
- Authors
- Keilmann, F., Gohle, C., & Holzwarth, R.
- Affiliations
- Max Planck Society (DE)
- Venue
- Optics Letters
- Publisher
- Optica Publishing Group
- Published
- 2004-07-01
- Volume
- 29
- Issue
- 13
- Pages
- 1542
- ISSN
- 0146-9592 (ISSN-L)
- 1539-4794
- OpenAlex
- W1979221508
- Cited by
- 734
- References
- 10
- Citations by year
- 2026: 22 · 2025: 26 · 2024: 26 · 2023: 50 · 2022: 29 · 2021: 51 · 2020: 56 · 2019: 43 · 2018: 62 · 2017: 40 · 2016: 60 · 2015: 38 · 2014: 41 · 2013: 33 · 2012: 29
- FWCI
- 4.75
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Optics Letters (publishedVersion)
- PubMed (publishedVersion)
- Max Planck Institute for Plasma Physics (submittedVersion)
- MPG.PuRe (Max Planck Society) (submittedVersion)
- Topics
- Physical Sciences › Chemistry › Spectroscopy › Spectroscopy and Laser Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Advanced Fiber Laser Technologies
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Keywords
- time-domain interferometry, mid-infrared spectroscopy, Fourier transform infrared spectrometer, femtosecond pulse trains, Ti:sapphire laser, terahertz spectroscopy
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Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
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