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Time-domain mid-infrared frequency-comb spectrometer
Abstract
A novel type of Fourier-transform infrared spectrometer (FTIR) is demonstrated. It is based on two Ti:sapphire lasers emitting femtosecond pulse trains with slightly different repetition frequencies. Two mid-infrared beams-derived from those lasers by rectification in GaSe-are superimposed upon a detector to produce purely time-domain interferograms that encode the infrared spectrum. The advantages of this spectrometer compared with the common FTIR include ease of operation (no moving parts), speed of acquisition (100 micros demonstrated), and not-yet-shown collimated long-distance propagation, diffraction-limited microscopic probing, and electronically controllable chemometric factoring. Extending time-domain frequency-comb spectroscopy to lower (terahertz) or higher (visible, ultraviolet) frequencies should be feasible.
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Holzner, S. (2015) · Elektronische Hochschulschriften der LMU München (Ludwig-Maximilians-Universität München) · doi:10.5282/edoc.18996
Chun, B. J., Kim, Y., & Kim, S. (2016) · Proceedings of SPIE, the International Society for Optical Engineering/Proceedings of SPIE · doi:10.1117/12.2212838
Rapid, High Resolution Frequency Comb Measurements
Coddington, I. R., Giorgetta, F. R., Baumann, E., Swann, W. C., & Newbury, N. R. (2011) · Advances in Optical Materials · doi:10.1364/assp.2011.ame1
Spectroscopic Sensing with Laser Frequency Combs
Picqué, N. (2014) · Advanced Photonics · doi:10.1364/sensors.2014.seth4c.1
Dual Comb Spectroscopy – Static Fourier transform spectroscopy with frequency combs
Bernhardt, B., Ideguchi, T., Holzner, S., Guelachvili, G., Hänsch, T. W., & Picqué, N. (2015) · Fourier Transform Spectroscopy/ Hyperspectral Imaging and Sounding of the Environment · doi:10.1364/fts.2015.fm2a.1
High Resolution Frequency Comb Molecular Spectroscopy
Coddington, I. R., Zolot, A. M., Baumann, E., Giorgetta, F. R., Rieker, G. B., Nicholson, J. W., Swann, W. C., & Newbury, N. R. (2013) · OSA Light, Energy and the Environment Congress · doi:10.1364/e2.2013.et2a.1
Dual-Comb Spectroscopy with Difference-Frequency-Generated Mid-Infrared Frequency Combs
Maser, D. L., Cruz, F. C., Ycas, G. G., Johnson, T., Klose, A., Giorgetta, F. R., Sinclair, L. C., Coddington, I. R., Newbury, N. R., & Diddams, S. A. (2015) · Frontiers in Optics · doi:10.1364/fio.2015.ftu2e.3
Molecular Spectroscopy with Two Laser Frequency Combs: From Vibrational to Doppler-Free Resolution
Picqué, N. (2015) · Frontiers in Optics · doi:10.1364/ls.2015.ltu5g.4
Efficient Two-Comb Fourier SpectroscopyPreprint
Mandon, J., Guelachvili, G., & Picqué, N. (2008) · arXiv (Cornell University)
Performance of a Coherent Dual Frequency Comb Spectrometer
Newbury, N. R., Baumann, E., Coddington, I. R., Giorgetta, F. R., Swann, W. C., & Zolot, A. M. (2011) · Imaging and Applied Optics · doi:10.1364/fts.2011.fthb2
Adler, F., Cossel, K. C., Thorpe, M. J., & Ye, J. (2009) · Advances in Optical Sciences Congress · doi:10.1364/nlo.2009.ntha3
Metadata
- Authors
- Keilmann, F., Gohle, C., & Holzwarth, R.
- Affiliations
- Max Planck Society (DE)
- Venue
- Optics Letters
- Publisher
- Optica Publishing Group
- Published
- 2004-07-01
- Volume
- 29
- Issue
- 13
- Pages
- 1542
- ISSN
- 0146-9592 (ISSN-L)
- 1539-4794
- OpenAlex
- W1979221508
- Cited by
- 734
- References
- 10
- Citations by year
- 2026: 22 · 2025: 26 · 2024: 26 · 2023: 50 · 2022: 29 · 2021: 51 · 2020: 56 · 2019: 43 · 2018: 62 · 2017: 40 · 2016: 60 · 2015: 38 · 2014: 41 · 2013: 33 · 2012: 29
- FWCI
- 4.75
- Type
- journal article
- Language
- en
- Open access
- closed
- Locations
- Optics Letters (publishedVersion)
- PubMed (publishedVersion)
- Max Planck Institute for Plasma Physics (submittedVersion)
- MPG.PuRe (Max Planck Society) (submittedVersion)
- Topics
- Physical Sciences › Chemistry › Spectroscopy › Spectroscopy and Laser Applications
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Advanced Fiber Laser Technologies
- Physical Sciences › Physics and Astronomy › Atomic and Molecular Physics, and Optics › Laser-Matter Interactions and Applications
- Keywords
- time-domain interferometry, mid-infrared spectroscopy, Fourier transform infrared spectrometer, femtosecond pulse trains, Ti:sapphire laser, terahertz spectroscopy
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