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Temperature-dependent excitonic photoluminescence excited by two-photon absorption in perovskite CsPbBr_3 quantum dots
Open accessAbstract
Recently, lead halide perovskite quantum dots have been reported with potential for photovoltaic and optoelectronic applications due to their excellent luminescent properties. Herein excitonic photoluminescence (PL) excited by two-photon absorption in perovskite CsPbBr3 quantum dots (QDs) has been studied at a broad temperature range, from 80 to 380 K. Two-photon absorption has been investigated and the absorption coefficient is up to 0.085 cm/GW at room temperature. Moreover, the PL spectrum excited by two-photon absorption shows a linear blue-shift (0.32 meV/K) below the temperature of 220 K. However, for higher temperatures, the PL peak approaches a roughly constant value and shows temperature-independent chromaticity up to 380 K. This behavior is distinct from the general red-shift for semiconductors and can be attributed to the result of thermal expansion, electron–phonon interaction and structural phase transition around 360 K. The strong nonlinear absorption and temperature-independent chromaticity of CsPbBr3 QDs observed in temperature range from 220 to 380 K will offer new opportunities in nonlinear photonics, light-harvesting, and light-emitting devices.
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Cites
Akkerman, Q. A., D’Innocenzo, V., Accornero, S., Scarpellini, A., Petrozza, A., Prato, M., & Manna, L. (2015) · Journal of the American Chemical Society · doi:10.1021/jacs.5b05602 · Cited by 2,197
Bright, multicoloured light-emitting diodes based on quantum dots
Sun, Q., Wang, Y. A., Li, L. S., Wang, D., Zhu, T., Xu, J., Yang, C., & Li, Y. (2007) · Nature Photonics · doi:10.1038/nphoton.2007.226 · Cited by 1,147
Cited by
van der Stam, W., Geuchies, J. J., Altantzis, T., van den Bos, K. H. W., Meeldijk, J. D., Van Aert, S., Bals, S., Vanmaekelbergh, D., & de Mello Donega, C. (2017) · Journal of the American Chemical Society · doi:10.1021/jacs.6b13079 · Cited by 732
Halide Perovskites for Nonlinear Optics
Xu, J., Li, X., Xiong, J., Yuan, C., Semin, S., Rasing, T., & Bu, X. (2020) · Advanced Materials · doi:10.1002/adma.201806736 · Cited by 355
Temperature-Dependent Optical Band Gap in CsPbBr3, MAPbBr3, and FAPbBr3 Single Crystals
Mannino, G., Deretzis, I., Smecca, E., La Magna, A., Alberti, A., Ceratti, D., & Cahen, D. (2020) · The Journal of Physical Chemistry Letters · doi:10.1021/acs.jpclett.0c00295 · Cited by 355
Metadata
- Authors
- Wei, K., Xu, Z., Chen, R., Zheng, X., Cheng, X., & Jiang, T.
- Venue
- Optics Letters
- Publisher
- Optica Publishing Group
- Published
- 2016-08-09
- Volume
- 41
- Issue
- 16
- Pages
- 3821
- ISSN
- 0146-9592 (ISSN-L)
- 1539-4794
- OpenAlex
- W2436072914
- Cited by
- 325
- References
- 2
- FWCI
- 14.03
- Type
- journal article
- Language
- en
- Open access
- green
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- Wei, K., Xu, Z., Chen, R., Zheng, X., Cheng, X., & Jiang, T. (2016). Temperature-dependent excitonic photoluminescence excited by two-photon absorption in perovskite CsPbBr_3 quantum dots. Optics Letters. https://doi.org/10.1364/ol.41.003821
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