Interfaces Between Cathode and Electrolyte in Solid State Lithium Batteries: Challenges and Perspectives

Nie, Kaihui; Hong, Yanshuai; Qiu, Jiliang; Li, Qinghao; Yu, Xiqian; Li, Hong; Chen, Liquan

doi:10.3389/fchem.2018.00616

Cited by 278Advanced Battery Materials and TechnologiesAdvancements in Battery MaterialsBattery Modeling and Management

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Interfaces Between Cathode and Electrolyte in Solid State Lithium Batteries: Challenges and Perspectives

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Nie, Kaihui, Hong, Yanshuai, Qiu, Jiliang, Li, Qinghao, Yu, Xiqian, Li, Hong, Chen, Liquan·2018·Frontiers in Chemistry

DOI 10.3389/fchem.2018.00616PMC PMC6299818

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Abstract

Solid state lithium batteries are widely accepted as promising candidates for next generation of various energy storage devices with the probability to realize improved energy density and superior safety performances. However, the interface between electrode and solid electrolyte remain a key issue that hinders practical development of solid state lithium batteries. In this review, we specifically focus on the interface between solid electrolytes and prevailing cathodes. The basic principles of interface layer formation are summarized and three kinds of interface layers can be categorized. For typical solid state lithium batteries, a most common and daunting challenge is to achieve and sustain intimate solid-solid contact. Meanwhile, different specific issues occur on various types of solid electrolytes, depending on the intrinsic properties of adjacent solid components. Our discussion mostly involves following electrolytes, including solid polymer electrolyte, inorganic solid oxide and sulfide electrolytes as well as composite electrolytes. The effective strategies to overcome the interface instabilities are also summarized. In order to clarify interfacial behaviors fundamentally, advanced characterization techniques with time, and atomic-scale resolution are required to gain more insights from different perspectives. And recent progresses achieved from advanced characterization are also reviewed here. We highlight that the cooperative characterization of diverse advanced characterization techniques is necessary to gain the final clarification of interface behavior, and stress that the combination of diverse interfacial modification strategies is required to build up decent cathode-electrolyte interface for superior solid state lithium batteries.

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Solid-state electrolytes allow the thickness of microbatteries to be reduced to micrometers.
“A significant advancement in this area has been the development of solid-state electrolytes, allowing the thickness of these microbatteries to be reduced to mere micrometers.”
From Comparative analysis of energy transfer mechanisms for neural implants (2024) · cites this paper as Nie et al., 2018
The Introduction discusses solid electrolytes’ conductivity, and the solid-oxide-electrolyte section discusses thin interfacial layers, but neither gives a thickness for microbatteries. Searches for microbatteries, micrometers, and battery thickness found no passage saying that solid-state electrolytes reduce microbattery thickness to micrometers. (LLM, conf=0.72)
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Authors: Nie, K., Hong, Y., Qiu, J., Li, Q., Yu, X., Li, H., & Chen, L.
Affiliations: Chinese Academy of Sciences (CN)
Corresponding author: Li, Qinghao
Yu, Xiqian
ORCID: Li, Qinghao
Yu, Xiqian
Li, Hong
Chen, Liquan
Venue: Frontiers in Chemistry
Publisher: Frontiers Media SA
Published: 2018-12-12
Volume: 6
Pages: 616-616
ISSN: 2296-2646 (ISSN-L)
DOI: 10.3389/fchem.2018.00616
PMC: PMC6299818
OpenAlex: W2903697882
Cited by: 278
References: 119
Citations by year: 2026: 32 · 2025: 39 · 2024: 33 · 2023: 42 · 2022: 42 · 2021: 42 · 2020: 34 · 2019: 14
FWCI: 1.25
Type: journal article
Language: en
Open access: gold
doi.org
Licence: cc-by
creativecommons.org/licenses/by/4.0/ (unspecified)
Locations: Frontiers in Chemistry (publishedVersion, cc-by)
Europe PMC (PubMed Central) (publishedVersion, cc-by)
PubMed Central (publishedVersion, cc-by)
PubMed (publishedVersion)
DOAJ (DOAJ: Directory of Open Access Journals) (submittedVersion)
Funders: National Natural Science Foundation of China (51822211)
eijing Municipal Science & Technology (Z171100000917021)
Topics: Physical Sciences › Engineering › Electrical and Electronic Engineering › Advanced Battery Materials and Technologies
Physical Sciences › Engineering › Electrical and Electronic Engineering › Advancements in Battery Materials
Physical Sciences › Engineering › Automotive Engineering › Battery Modeling and Management
Keywords: solid-state lithium batteries, cathode-electrolyte interface, solid-solid contact, solid polymer electrolytes, solid oxide electrolytes, composite electrolytes, interfacial instability

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Interfaces Between Cathode and Electrolyte in Solid State Lithium Batteries: Challenges and Perspectives

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