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Heterogeneous Catalyst Deactivation and Regeneration: A Review
Open accessAbstract
Deactivation of heterogeneous catalysts is a ubiquitous problem that causes loss of catalytic rate with time. This review on deactivation and regeneration of heterogeneous catalysts classifies deactivation by type (chemical, thermal, and mechanical) and by mechanism (poisoning, fouling, thermal degradation, vapor formation, vapor-solid and solid-solid reactions, and attrition/crushing). The key features and considerations for each of these deactivation types is reviewed in detail with reference to the latest literature reports in these areas. Two case studies on the deactivation mechanisms of catalysts used for cobalt Fischer-Tropsch and selective catalytic reduction are considered to provide additional depth in the topics of sintering, coking, poisoning, and fouling. Regeneration considerations and options are also briefly discussed for each deactivation mechanism.
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Citations
Cited by
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Li, D., Xu, F., Tang, X., Dai, S., Pu, T., Liu, X., Tian, P., Xuan, F., Xu, Z., Wachs, I. E., et al. (2022) · Nature Catalysis · doi:10.1038/s41929-021-00729-4 · Cited by 519
Pyrolysis technology for plastic waste recycling: A state-of-the-art review
Dai, L., Zhou, N., Lv, Y., Cheng, Y., Wang, Y., Liu, Y., Cobb, K., Chen, P., Lei, H., & Ruan, R. (2022) · Progress in Energy and Combustion Science · doi:10.1016/j.pecs.2022.101021 · Cited by 485
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Rey, J. R. C., Longo, A., Rijo, B., Pedrero, C. M., Tarelho, L. A. C., Brito, P. S. D., & Nobre, C. (2024) · Fuel · doi:10.1016/j.fuel.2024.132776 · Cited by 149
Metadata
- Authors
- Argyle, M., & Bartholomew, C.
- Venue
- Catalysts
- Publisher
- MDPI AG
- Published
- 2015-02-26
- Volume
- 5
- Issue
- 1
- Pages
- 145-269
- ISSN
- 2073-4344 (ISSN-L)
- OpenAlex
- W2093771834
- Cited by
- 1,862
- References
- 0
- FWCI
- 32.21
- Type
- journal article
- Language
- en
- Open access
- gold
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