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Electrocarboxylation: towards sustainable and efficient synthesis of valuable carboxylic acids
Open accessAbstract
The near-unlimited availability of CO 2 has stimulated a growing research effort in creating value-added products from this greenhouse gas. This paper presents the trends on the most important methods used in the electrochemical synthesis of carboxylic acids from carbon dioxide. An overview is given of different substrate groups which form carboxylic acids upon CO 2 fixation, including mechanistic considerations. While most work focuses on the electrocarboxylation of substrates with sacrificial anodes, this review considers the possibilities and challenges of implementing other synthetic methodologies. In view of potential industrial application, the choice of reactor setup, electrode type and reaction pathway has a large influence on the sustainability and efficiency of the process.
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Recent advances in catalytic hydrogenation of carbon dioxide
Wang, W., Wang, S., Ma, X., & Gong, J. (2011) · Chemical Society Reviews · doi:10.1039/c1cs15008a · Cited by 3,316
Cited by
Electrode Materials in Modern Organic Electrochemistry
Heard, D. M., & Lennox, A. J. J. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.202005745 · Cited by 523
Carbon capture and utilization technologies: a literature review and recent advances
Baena-Moreno, F. M., Rodríguez-Galán, M., Vega, F., Alonso-Fariñas, B., Vilches Arenas, L. F., & Navarrete, B. (2019) · Energy Sources, Part A: Recovery, Utilization, and Environmental Effects · doi:10.1080/15567036.2018.1548518 · Cited by 351
Direct electrochemical defluorinative carboxylation of α-CF 3 alkenes with carbon dioxide
Gao, X.-T., Zhang, Z., Wang, X., Tian, J.-S., Xie, S.-L., Zhou, F., & Zhou, J. (2020) · Chemical Science · doi:10.1039/d0sc04091f · Cited by 142
Metadata
- Authors
- Matthessen, R., Fransaer, J., Binnemans, K., & De Vos, D. E.
- Venue
- Beilstein Journal of Organic Chemistry
- Publisher
- Beilstein Institut
- Published
- 2014-10-27
- Volume
- 10
- Pages
- 2484-2500
- ISSN
- 1860-5397 (ISSN-L)
- OpenAlex
- W2156803765
- Cited by
- 197
- References
- 1
- FWCI
- 2.14
- Type
- journal article
- Language
- en
- Open access
- diamond
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- Matthessen, R., Fransaer, J., Binnemans, K., & De Vos, D. E. (2014). Electrocarboxylation: towards sustainable and efficient synthesis of valuable carboxylic acids. Beilstein Journal of Organic Chemistry. https://doi.org/10.3762/bjoc.10.260
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