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An overview of current issues in the uptake of atmospheric trace gases by aerosols and clouds
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Abstract
Abstract. A workshop was held in the framework of the ACCENT (Atmospheric Composition Change – a European Network) Joint Research Programme on "Aerosols" and the Programme on "Access to Laboratory Data". The aim of the workshop was to hold "Gordon Conference" type discussion covering accommodation and reactive uptake of water vapour and trace pollutant gases on condensed phase atmospheric materials. The scope was to review and define the current state of knowledge of accommodation coefficients for water vapour on water droplet and ice surfaces, and uptake of trace gas species on a variety of different surfaces characteristic of the atmospheric condensed phase particulate matter and cloud droplets. Twenty-six scientists participated in this meeting through presentations, discussions and the development of a consensus review. In this review we present an analysis of the state of knowledge on the thermal and mass accommodation coefficient for water vapour on aqueous droplets and ice and a survey of current state-of the-art of reactive uptake of trace gases on a range of liquid and solid atmospheric droplets and particles. The review recommends consistent definitions of the various parameters that are needed for quantitative representation of the range of gas/condensed surface kinetic processes important for the atmosphere and identifies topics that require additional research.
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Metadata
- Authors
- Kolb, C. E., Cox, R. A., Abbatt, J. P. D., Ammann, M., Davis, E. J., Donaldson, D. J., Garrett, B. C., George, C., Griffiths, P. T., Hanson, D. R., Kulmala, M., McFiggans, G., Pöschl, U., Riipinen, I., Rossi, M. J., Rudich, Y., Wagner, P. E., Winkler, P. M., Worsnop, D. R., & O' Dowd, C. D.
- Affiliations
- Aerodyne Research (US)
- University of Cambridge (GB)
- University of Toronto (CA)
- Paul Scherrer Institute (CH)
- University of Washington (US)
- Pacific Northwest National Laboratory (US)
- Centre National de la Recherche Scientifique (FR)
- Augsburg University (US)
- University of Helsinki (FI)
- University of Manchester (GB)
- Max Planck Institute for Chemistry (DE)
- Weizmann Institute of Science (IL)
- University of Vienna (AT)
- NSF National Center for Atmospheric Research (US)
- ORCID
- Venue
- Atmospheric Chemistry and Physics
- Publisher
- Copernicus GmbH
- Published
- 2010-11-10
- Volume
- 10
- Issue
- 21
- Pages
- 10561-10605
- ISSN
- 1680-7316 (ISSN-L)
- 1680-7324
- OpenAlex
- W2164562420
- Cited by
- 405
- References
- 420
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- FWCI
- 18.25
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- journal article
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- en
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- ARAN (University of Galway Research Repository) (Ollscoil na Gaillimhe – University of Galway) (submittedVersion, cc-by-nc)
- Research Repository UCD (University College Dublin) (cc-by-nc)
- Funders
- European Commission
- Topics
- Physical Sciences › Earth and Planetary Sciences › Atmospheric Science › Atmospheric chemistry and aerosols
- Physical Sciences › Environmental Science › Global and Planetary Change › Atmospheric aerosols and clouds
- Physical Sciences › Chemical Engineering › Fluid Flow and Transfer Processes › Advanced Combustion Engine Technologies
- Keywords
- cloud droplets, thermal accommodation coefficient, mass accommodation coefficient, aqueous droplets, ice surfaces, atmospheric aerosols, atmospheric composition change
About these checks
Registry, retraction, Cites and statistics results are computed, not judged, with one exception: a printed reference that no index lists is read once by a model before it counts as a citation error. Claims are extracted by a model and kept only when their quote appears verbatim in the text; each cited source is then checked, with a model’s help, for whether it says what the claim relies on. Those verdicts can be wrong — read the claim’s quote and the cited source before relying on one.
Statistics and arithmetic are recomputed, not judged.
Confidence bands are shown only for fields calibrated on our annotated test set. None is calibrated yet, so no band is shown.
What counts as a claim ›How we measure confidence ›How we check this ›
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