The DOI matches its Crossref record; 55 of the 55 references it cites were found in a registry or an index.
Laboratory investigation of photochemical oxidation of organic aerosol from wood fires 1: measurement and simulation of organic aerosol evolution
Open accessAbstract
Abstract. Experiments were conducted to investigate the effects of photo-oxidation on organic aerosol (OA) emissions from flaming and smoldering hard- and soft-wood fires under plume-like conditions. This was done by exposing the dilute emissions from a small wood stove to UV light in a smog chamber and measuring the gas- and particle-phase pollutant concentrations with a suite of instruments including a Proton Transfer Reaction Mass Spectrometer (PTR-MS), an Aerosol Mass Spectrometer (AMS) and a thermodenuder. The measurements highlight how atmospheric processing can lead to considerable evolution of the mass and volatility of biomass-burning OA. Photochemical oxidation produced substantial new OA, increasing concentrations by a factor of 1.5 to 2.8 after several hours of exposure to typical summertime hydroxyl radical (OH) concentrations. Less than 20% of this new OA could be explained using a state-of-the-art secondary organic aerosol model and the measured decay of traditional SOA precursors. The thermodenuder data indicate that the primary OA is semivolatile; at 50°C between 50 and 80% of the fresh primary OA evaporated. Aging reduced the volatility of the OA; at 50°C only 20 to 40% of aged OA evaporated. The predictions of a volatility basis-set model that explicitly tracks the partitioning and aging of low-volatility organics was compared to the chamber data. The OA production can be explained by the oxidation of low-volatility organic vapors; the model can also reproduce observed changes in OA volatility and composition. The model was used to investigate the competition between photochemical processing and dilution on OA concentrations in plumes.
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Cites
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Minguillón, M. C., Perron, N., Querol, X., Szidat, S., Fahrni, S. M., Alastuey, A., Jimenez, J. L., Mohr, C., Ortega, A. M., Day, D. A., et al. (2011) · Atmospheric Chemistry and Physics · doi:10.5194/acp-11-12067-2011 · Cited by 153
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Metadata
- Authors
- Grieshop, A. P., Logue, J. M., Donahue, N. M., & Robinson, A. L.
- Venue
- Atmospheric Chemistry and Physics
- Publisher
- Copernicus GmbH
- Published
- 2009-02-18
- Volume
- 9
- Issue
- 4
- Pages
- 1263-1277
- ISSN
- 1680-7316 (ISSN-L)
- 1680-7324
- OpenAlex
- W2158129017
- Cited by
- 417
- References
- 55
- FWCI
- 22.86
- Type
- journal article
- Language
- en
- Open access
- gold
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