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Efficient TiO2 Photocatalysts from Surface Hybridization of TiO2 Particles with Graphite‐like Carbon
Abstract
Surface hybridization of TiO 2 with graphite‐like carbon layers of a few molecular layers thickness yields efficient photocatalysts. Photoelectrochemical measurements confirm an electronic interaction between TiO 2 and the graphite‐like carbon. A TiO 2 photocatalyst with a carbon shell of three molecular layers thickness (∼1 nm) shows the highest photocatalytic activity which is about two times higher than that of Degussa P25 TiO 2 under UV light irradiation. The mechanism of the enhanced photocatalytic activity under UV irradiation is based on the high migration efficiency of photoinduced electrons at the graphite‐like carbon/TiO 2 interface, which is due to the electronic interaction between both materials. In addition, a high activity under visible light irradiation is observed after graphite‐like carbon hybridization. TiO 2's response is extended into the visible range of the solar spectrum due to the electronic coupling of π states of the graphite‐like carbon and conduction band states of TiO 2.
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Environmental applications of semiconductor photocatalysis
Hoffmann, M. R., Martin, S. T., Choi, W., & Bahnemann, D. W. (1995) · Chemical Reviews · doi:10.1021/cr00033a004 · Cited by 18,495
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Cited by
Zhou, Y., Bao, Q., Tang, L. A. L., Zhong, Y., & Loh, K. P. (2009) · Chemistry of Materials · doi:10.1021/cm9006603 · Cited by 1,542
A review of TiO2 nanoparticles
Gupta, S. M., & Tripathi, M. (2011) · Chinese Science Bulletin · doi:10.1007/s11434-011-4476-1 · Cited by 1,270
Ming, H., Ma, Z., Liu, Y., Pan, K., Yu, H., Wang, F., & Kang, Z. (2012) · Dalton Transactions · doi:10.1039/c2dt30985h · Cited by 819
Mesoporous Anatase Titania Hollow Nanostructures though Silica‐Protected Calcination
Joo, J. B., Zhang, Q., Lee, I., Dahl, M., Zaera, F., & Yin, Y. (2012) · Advanced Functional Materials · doi:10.1002/adfm.201101927 · Cited by 433
Su, T., Peng, R., Hood, Z. D., Naguib, M., Ivanov, I. N., Keum, J. K., Qin, Z., Guo, Z., & Wu, Z. (2018) · ChemSusChem · doi:10.1002/cssc.201702317 · Cited by 426
Metadata
- Authors
- Zhang, L., Fu, H., & Zhu, Y.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2008-08-06
- Volume
- 18
- Issue
- 15
- Pages
- 2180-2189
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2068845033
- Cited by
- 797
- References
- 2
- FWCI
- 17.16
- Type
- journal article
- Language
- en
- Open access
- closed
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- Zhang, L., Fu, H., & Zhu, Y. (2008). Efficient TiO2 Photocatalysts from Surface Hybridization of TiO2 Particles with Graphite‐like Carbon. Advanced Functional Materials. https://doi.org/10.1002/adfm.200701478
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