Cited by 178Electrocatalysts for Energy ConversionAdvanced Photocatalysis Techniques2D Materials and Applications

A Novel MoSe2–Reduced Graphene Oxide/Polyimide Composite Film for Applications in Electrocatalysis and Photoelectrocatalysis Hydrogen Evolution

Jia, Lingpu, Sun, Xiao, Jiang, Yimin, Yu, Shenjiao, Wang, Chunming·2015·Advanced Functional Materials

Abstract

Promising catalytic activity of MoSe2 in the hydrogen evolution reaction (HER) is synthesized on a new reduced graphene oxide/polyimide (rGO/PI) substrate by a simple electrochemical method. The MoSe2 nanoparticles have excellent photo‐responsive properties; the potential difference could reach 0.45 V with the photo‐responsive time just 0.6 s. Furthermore, MoSe2 thin film exhibits superior catalytic activity in the hydrogen evolution reaction (HER). It has a greater cathode current at more positive potential compared to other MoSe2 and MoS2, and the efficiency of H2 evolution is strongly influenced by illumination; this suggests that MoSe2 composite film has good photoelectrocatalysis properties for hydrogen evolution. Besides, both dark and illumination MoSe2 films exhibit extremely high stability in acidic solution as the HER catalytic activity shows no degradation after 100 cycles for two hours. All results indicate that MoSe2–rGO/PI composite film has potential to be a better catalyst for HER.

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Crossref · 10.1002/adfm.201401814

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Authors
Jia, L., Sun, X., Jiang, Y., Yu, S., & Wang, C.
Affiliations
Lanzhou University (CN)
Corresponding author
Wang, Chunming
Venue
Advanced Functional Materials
Publisher
Wiley
Published
2014-09-05
Volume
25
Issue
12
Pages
1814-1820
ISSN
  • 1616-301X (ISSN-L)
  • 1616-3028
OpenAlex
W2086512413
Cited by
178
References
42
Citations by year
2025: 3 · 2024: 14 · 2023: 12 · 2022: 7 · 2021: 11 · 2020: 17 · 2019: 22 · 2018: 23 · 2017: 29 · 2016: 25 · 2015: 14
FWCI
7.47
Type
journal article
Language
en
Open access
closed
Locations
  • Advanced Functional Materials (publishedVersion)
  • Lanzhou University Institutional Repository (submittedVersion)
Topics
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
  • Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
  • Physical Sciences › Materials Science › Materials Chemistry › 2D Materials and Applications
Keywords
MoSe2, reduced graphene oxide, polyimide, composite films, hydrogen evolution reaction, photoelectrocatalysis, electrocatalysis, electrochemical synthesis, photoresponsivity, catalyst stability, acidic media

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