A CNT@MoSe 2 hybrid catalyst for efficient and stable hydrogen evolution

Huang, Yunpeng; Lu, Hengyi; Gu, Huahao; Fu, Jun; Mo, Shuyi; Wei, Chun; Miao, Yue-E; Liu, Tianxi

doi:10.1039/c5nr05739f

Cited by 167Electrocatalysts for Energy ConversionCO2 Reduction Techniques and CatalystsAdvanced Photocatalysis Techniques

A CNT@MoSe 2 hybrid catalyst for efficient and stable hydrogen evolution

Huang, Yunpeng, Lu, Hengyi, Gu, Huahao, Fu, Jun, Mo, Shuyi, Wei, Chun, Miao, Yue-E, Liu, Tianxi·2015·Nanoscale

DOI 10.1039/c5nr05739f

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Abstract

Exploration of high-efficiency Pt-free electrochemical catalysts for hydrogen evolution reaction (HER) is considered as a great challenge for the development of sustainable and carbon dioxide free energy conversion systems. In this work, a unique hierarchical nanostructure of few-layered MoSe2 nanosheets perpendicularly grown on carbon nanotubes (CNTs) is synthesized through a one-step solvothermal reaction. This rationally designed architecture based on a highly conductive CNT substrate possesses fully exposed active edges and open structures for fast ion/electron transfer, thus leading to remarkable HER activity with a low onset potential of -0.07 V vs. RHE (reversible hydrogen electrode), a small Tafel slope of 58 mV per decade and excellent long-cycle stability. Therefore, this noble-metal-free and highly efficient catalyst enables prospective applications for industrial, renewable hydrogen production.

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Integration of MoSe2 with carbon substrates like CNTs, graphene, carbon fiber cloth, or cotton-derived carbon fiber aerogel promotes its catalytic performance.
“Several reports have proved that the integration of MoSe2 with carbon substrates like carbon nanotubes,10 graphene,11,12 carbon fiber cloth13 or cotton-derived carbon fiber aerogel14 could promote its catalytic performance.”
From Carbon-Nanotube-Incorporated Graphene Scroll-Sheet Conjoined Aerogels for Efficient Hydrogen Evolution Reaction (2017) · cites this paper as [10]

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Authors: Huang, Y., Lu, H., Gu, H., Fu, J., Mo, S., Wei, C., Miao, Y.-E., & Liu, T.
Affiliations: Fudan University (CN)
Guilin University of Technology (CN)
Donghua University (CN)
Corresponding author: Miao, Yue-E
Liu, Tianxi
ORCID: Huang, Yunpeng
Lu, Hengyi
Mo, Shuyi
Wei, Chun
Miao, Yue-E
Liu, Tianxi
Venue: Nanoscale
Publisher: Royal Society of Chemistry (RSC)
Published: 2015
Volume: 7
Issue: 44
Pages: 18595-18602
ISSN: 2040-3364 (ISSN-L)
2040-3372
DOI: 10.1039/c5nr05739f
OpenAlex: W1843185883
Cited by: 167
References: 35
Citations by year: 2026: 4 · 2025: 2 · 2024: 6 · 2023: 6 · 2022: 12 · 2021: 10 · 2020: 23 · 2019: 29 · 2018: 35 · 2017: 24 · 2016: 16
FWCI: 7.40
Type: journal article
Language: en
Open access: closed
Locations: Nanoscale (publishedVersion)
PubMed (publishedVersion)
Funders: National Natural Science Foundation of China
Natural Science Foundation of Guangxi Province
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Advanced Photocatalysis Techniques
Keywords: hydrogen evolution reaction, carbon nanotubes, MoSe2 nanosheets, platinum-free electrocatalysts, hierarchical nanostructures, solvothermal synthesis, hydrogen production, catalyst stability

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A CNT@MoSe 2 hybrid catalyst for efficient and stable hydrogen evolution

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