The DOI matches its Crossref record; 5 of the 5 references it cites were found in a registry or an index.
Oriented Growth of ZIF‐67 to Derive 2D Porous CoPO Nanosheets for Electrochemical‐/Photovoltage‐Driven Overall Water Splitting
Abstract
Hydrogen generation from water splitting driven by electric/solar energy is highly desirable, which requires efficient and robust bifunctional electrocatalysts for both hydrogen and oxygen evolution reactions. 2D porous hybrids with attractive chemical and structural properties are the first‐class candidates for water splitting, while control over efficient and modulable synthesis remains a huge challenge. This work demonstrates a zeolitic imidazolate framework‐67 (ZIF‐67) nanoplate self‐template approach to fabricate 2D porous oxygen‐incorporated cobalt phosphide (CoPO) ultrathin nanosheets. The synthesis starts with the oriented growth of ZIF‐67 nanoplates along [211] crystal plane, followed by oxidation/phosphorization processes for pore generation and O/P coincorporation in the hybrid. The resultant 2D porous CoPO nanosheets afford very small voltages of 1.52 and 1.98 V for overall water splitting at 10 and 200 mA cm−2, respectively. This excellent bifunctionality further provides the basis for photovoltage‐driven water splitting at a Faradaic efficiency of 97.6%. These findings offer a general strategy for rational design and modulation of 2D porous catalysts for various electrocatalytic and other applications.
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Cites
Electrocatalysis for the oxygen evolution reaction: recent development and future perspectives
Suen, N.-T., Hung, S.-F., Quan, Q., Zhang, N., Xu, Y.-J., & Chen, H. M. (2017) · Chemical Society Reviews · doi:10.1039/c6cs00328a · Cited by 6,307
Nanostructured Nickel Phosphide as an Electrocatalyst for the Hydrogen Evolution Reaction
Popczun, E. J., McKone, J. R., Read, C. G., Biacchi, A. J., Wiltrout, A. M., Lewis, N. S., & Schaak, R. E. (2013) · Journal of the American Chemical Society · doi:10.1021/ja403440e · Cited by 2,911
Enhanced catalytic activity in strained chemically exfoliated WS2 nanosheets for hydrogen evolution
Voiry, D., Yamaguchi, H., Li, J., Silva, R., Alves, D. C. B., Fujita, T., Chen, M., Asefa, T., Shenoy, V. B., Eda, G., et al. (2013) · Nature Materials · doi:10.1038/nmat3700 · Cited by 2,641
Tian, J., Liu, Q., Asiri, A. M., & Sun, X. (2014) · Journal of the American Chemical Society · doi:10.1021/ja503372r · Cited by 2,373
Highly active hydrogen evolution catalysis from metallic WS 2 nanosheets
Lukowski, M. A., Daniel, A. S., English, C. R., Meng, F., Forticaux, A., Hamers, R. J., & Jin, S. (2014) · Energy Environ. Sci. · doi:10.1039/c4ee01329h · Cited by 709
Cited by
Bifunctional Electrocatalysts for Overall and Hybrid Water Splitting
Quan, L., Jiang, H., Mei, G., Sun, Y., & You, B. (2024) · Chemical Reviews · doi:10.1021/acs.chemrev.3c00332 · Cited by 874
Zhang, H., Maijenburg, A. W., Li, X., Schweizer, S. L., & Wehrspohn, R. B. (2020) · Advanced Functional Materials · doi:10.1002/adfm.202003261 · Cited by 666
Multifunctional Transition Metal‐Based Phosphides in Energy‐Related Electrocatalysis
Li, Y., Dong, Z., & Jiao, L. (2020) · Advanced Energy Materials · doi:10.1002/aenm.201902104 · Cited by 603
Gong, Y., Jiao, L., Qian, Y., Pan, C., Zheng, L., Cai, X., Liu, B., Yu, S., & Jiang, H. (2020) · Angewandte Chemie International Edition · doi:10.1002/anie.201914977 · Cited by 592
Porous Two-Dimensional Materials for Photocatalytic and Electrocatalytic Applications
Wang, H., Liu, X., Niu, P., Wang, S., Shi, J., & Li, L. (2020) · Matter · doi:10.1016/j.matt.2020.04.002 · Cited by 435
Metadata
- Authors
- Anandhababu, G., Huang, Y., Babu, D. D., Wu, M., & Wang, Y.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2018-01-09
- Volume
- 28
- Issue
- 9
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2783003019
- Cited by
- 199
- References
- 5
- FWCI
- 6.45
- Type
- journal article
- Language
- en
- Open access
- closed
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- Anandhababu, G., Huang, Y., Babu, D. D., Wu, M., & Wang, Y. (2018). Oriented Growth of ZIF‐67 to Derive 2D Porous CoPO Nanosheets for Electrochemical‐/Photovoltage‐Driven Overall Water Splitting. Advanced Functional Materials. https://doi.org/10.1002/adfm.201706120
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