The DOI matches its Crossref record; 56 of the 56 references it cites were found in a registry or an index.
Room‐Temperature Self‐Healing and Recyclable Tough Polymer Composites Using Nitrogen‐Coordinated Boroxines
Abstract
In this paper, nitrogen‐coordinated boroxines are exploited for the fabrication of self‐healing and recyclable polymer composites with enhanced mechanical properties. The 3D polymer networks cross‐linked with nitrogen‐coordinated boroxines are first synthesized through the trimerization of ortho‐aminomethyl‐phenylboronic acid groups at the terminals of poly(propylene glycol) (PPG) chains, and subsequently, the mechanically robust polymer composites are fabricated by utilizing the complexation of nitrogen‐coordinated boroxine‐containing PPG (N‐boroxine‐PPG) with poly(acrylic acid) (PAA) and hydrogen‐bonding interactions between them. The N‐boroxine‐PPG is soft with a tensile strength of 0.19 MPa, whereas the tensile strengths of N‐boroxine‐PPG/PAA composites can be tailored to range from 1.7 to 12.7 MPa by increasing the PAA contents in the polymer composites. It is revealed that the amine ligands can facilitate the formation and dissociation of nitrogen‐coordinated boroxines at room temperature. Moreover, the reversibility of nitrogen‐coordinated boroxines and hydrogen‐bonding interactions enable multiple cycles of healing and recycling of the damaged N‐boroxine‐PPG/PAA composites. The healed and recycled N‐boroxine‐PPG/PAA polymer composites regain most of their mechanical strength.
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Wang, X., Zhan, S., Lu, Z., Li, J., Yang, X., Qiao, Y., Men, Y., & Sun, J. (2020) · Advanced Materials · doi:10.1002/adma.202005759 · Cited by 575
Self-citationA Fast Room‐Temperature Self‐Healing Glassy Polyurethane
Xu, J., Chen, J., Zhang, Y., Liu, T., & Fu, J. (2021) · Angewandte Chemie International Edition · doi:10.1002/anie.202017303 · Cited by 375
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Zhang, X., Wang, S., Jiang, Z., Li, Y., & Jing, X. (2020) · Journal of the American Chemical Society · doi:10.1021/jacs.0c10244 · Cited by 363
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Metadata
- Authors
- Bao, C., Jiang, Y., Zhang, H., Lu, X., & Sun, J.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2018-04-19
- Volume
- 28
- Issue
- 23
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W2802146476
- Cited by
- 266
- References
- 56
- FWCI
- 13.62
- Type
- journal article
- Language
- en
- Open access
- closed
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