The DOI matches its Crossref record; 25 of the 25 references it cites were found in a registry or an index.
“Water‐in‐Deep Eutectic Solvent” Electrolytes for High‐Performance Aqueous Zn‐Ion Batteries
Abstract
Aqueous Zn‐ion batteries have been considered as promising alternatives to Li‐ion batteries due to their abundant reserves, low price, and high safety. However, Zn anode shows poor reversibility and cycling stability in most conventional aqueous electrolytes. Here, a new type of aqueous Zn‐ion electrolyte based on ZnCl 2–acetamide deep eutectic solvent with both environmental and economic friendliness has been prepared. The water molecule introduced in the “water‐in‐deep eutectic solvent” electrolyte could reduce the Zn 2+ desolvation energy barrier by regulating Zn 2+ solvation structure to promote uniform Zn nucleation. Zn anode shows improved electrochemical performance (≈98% Coulombic efficiency over 1000 cycles) in the electrolyte whose molar ratio of ZnCl 2:acetamide:H 2 O is 1:3:1. The assembled full battery composed of phenazine cathode and Zn anode could stably cycle over 10 000 cycles with a high capacity retention of 85.7%. Overall, this work offers new insights into exploring new green electrolyte systems for Zn‐ion batteries.
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Cites
Towards greener and more sustainable batteries for electrical energy storage
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Eutectic‐Based Ionic Liquids with Metal‐Containing Anions and Cations
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A ZnCl2 water-in-salt electrolyte for a reversible Zn metal anode
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Cited by
Liu, Z., Wang, R., Ma, Q., Wan, J., Zhang, S., Zhang, L., Li, H., Luo, Q., Wu, J., Zhou, T., et al. (2024) · Advanced Functional Materials · doi:10.1002/adfm.202214538 · Cited by 394
Electrolytes in Organic Batteries
Li, M., Hicks, R. P., Chen, Z., Luo, C., Guo, J., Wang, C., & Xu, Y. (2023) · Chemical Reviews · doi:10.1021/acs.chemrev.2c00374 · Cited by 303
Metadata
- Authors
- Shi, J., Sun, T., Bao, J., Zheng, S., Du, H., Li, L., Yuan, X., Ma, T., & Tao, Z.
- Venue
- Advanced Functional Materials
- Publisher
- Wiley
- Published
- 2021-04-15
- Volume
- 31
- Issue
- 23
- ISSN
- 1616-301X (ISSN-L)
- 1616-3028
- OpenAlex
- W3156782529
- Cited by
- 281
- References
- 25
- FWCI
- 12.17
- Type
- journal article
- Language
- en
- Open access
- closed
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- Shi, J., Sun, T., Bao, J., Zheng, S., Du, H., Li, L., Yuan, X., Ma, T., & Tao, Z. (2021). “Water‐in‐Deep Eutectic Solvent” Electrolytes for High‐Performance Aqueous Zn‐Ion Batteries. Advanced Functional Materials. https://doi.org/10.1002/adfm.202102035
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