Cited by 117Electrocatalysts for Energy ConversionCO2 Reduction Techniques and CatalystsFuel Cells and Related Materials

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Monolithic Ni‐Mo‐B Bifunctional Electrode for Large Current Water Splitting

Liu, Huixiang, Li, Xuanyang, Chen, Lulu, Zhu, Xiaodong, Dong, Pei, Chee, Mason Oliver Lam, Ye, Mingxin, Guo, Yanhui, Shen, Jianfeng·2022·Advanced Functional Materials

DOI 10.1002/adfm.202107308

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Abstract

Screening and developing highly efficient electrodes is key to large‐scale water electrolysis. The practical industrial electrode should fulfill several criteria of high activity, structural stability, and fast bubble evolution at a large current density. In this study, a novel monolithic 3D hollow foam electrode that can achieve the requirements of large current density water electrolysis is developed and fabricated through a simple electroless plating‐calcination strategy. This strong 3D Ni‐Mo‐B hollow foam electrode can withstand a pressure of 2.37 MPa and exhibits high electrochemical surface area, high conductivity, and low gas transfer resistance, drastically boosting its catalytic performance. It affords 50 mA cm –2 at overpotentials of only 68 mV for hydrogen evolution reaction and 293 mV for oxygen evolution reaction and can survive at a large current density of 5 A cm –2 while maintaining its structure and performance in 1.0 m KOH. The advantages of facile preparation, high mechanical strength, high gas mass transfer ability, and excellent performance enable this structure to be a potential electrode, active substrate, or 3D catalyst in many fields.

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Authors: Liu, H., Li, X., Chen, L., Zhu, X., Dong, P., Chee, M. O. L., Ye, M., Guo, Y., & Shen, J.
Affiliations: Fudan University (CN)
George Mason University (US)
Corresponding author: Ye, Mingxin
Guo, Yanhui
Shen, Jianfeng
ORCID: Liu, Huixiang
Li, Xuanyang
Chen, Lulu
Zhu, Xiaodong
Dong, Pei
Ye, Mingxin
Guo, Yanhui
Shen, Jianfeng
Venue: Advanced Functional Materials
Publisher: Wiley
Published: 2021-10-08
Volume: 32
Issue: 4
ISSN: 1616-301X (ISSN-L)
1616-3028
DOI: 10.1002/adfm.202107308
OpenAlex: W3207149998
Cited by: 117
References: 63
Citations by year: 2026: 11 · 2025: 17 · 2024: 34 · 2023: 39 · 2022: 15 · 2021: 1
FWCI: 4.18
Type: journal article
Language: en
Open access: closed
Licence: onlinelibrary.wiley.com/termsAndConditions#vor (vor)
Locations: Advanced Functional Materials (publishedVersion)
Funders: National Natural Science Foundation of China (51972064, 52172189)
Topics: Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › Electrocatalysts for Energy Conversion
Physical Sciences › Energy › Renewable Energy, Sustainability and the Environment › CO2 Reduction Techniques and Catalysts
Physical Sciences › Engineering › Electrical and Electronic Engineering › Fuel Cells and Related Materials
Keywords: bifunctional electrocatalysts, water electrolysis, hydrogen evolution reaction, oxygen evolution reaction, electroless plating, calcination, high current density, gas mass transfer, electrochemically active surface area, KOH electrolyte

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Monolithic Ni‐Mo‐B Bifunctional Electrode for Large Current Water Splitting

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